Modelling the relationship between liquid water content and cloud droplet number concentration observed in low clouds in the summer Arctic and its radiative effects

• Published in: Atmospheric Chemistry and Physics
• Main Authors: Dionne, Joelle, Salzen, Knut von, Cole, Jason, Mahmood, Rashed, Leaitch, W. Richard, Lesins, Glen, Folkins, Ian, Chang, Rachel
• Other Authors: Barcelona Supercomputing Center
• Format: Article in Journal/Newspaper
• Language: English
• Published: European Geoscience Union 2020
• Subjects: Àrees temàtiques de la UPC::Desenvolupament humà i sostenible::Degradació ambiental::Canvi climàtic; Climatic changes; Liquid water content; Cloud droplet number concentration; Summer Arctic; Canvis climàtics; Arctic; Canada; Resolute Bay
• Online Access: http://hdl.handle.net/2117/178812; https://doi.org/10.5194/acp-20-29-2020

Low clouds persist in the summer Arctic with important consequences for the radiation budget. In this study, we simulate the linear relationship between liquid water content (LWC) and cloud droplet number concentration (CDNC) observed during an aircraft campaign based out of Resolute Bay, Canada, conducted as part of the Network on Climate and Aerosols: Addressing Key Uncertainties in Remote Canadian Environments study in July 2014. Using a single-column model, we find that autoconversion can explain the observed linear relationship between LWC and CDNC. Of the three autoconversion schemes we examined, the scheme using continuous drizzle (Khairoutdinov and Kogan, 2000) appears to best reproduce the observed linearity in the tenuous cloud regime (Mauritsen et al., 2011), while a scheme with a threshold for rain (Liu and Daum, 2004) best reproduces the linearity at higher CDNC. An offline version of the radiative transfer model used in the Canadian Atmospheric Model version 4.3 is used to compare the radiative effects of the modelled and observed clouds. We find that there is no significant difference in the upward longwave cloud radiative effect at the top of the atmosphere from the three autoconversion schemes (p=0.05) but that all three schemes differ at p=0.05 from the calculations based on observations. In contrast, the downward longwave and shortwave cloud radiative effect at the surface for the Wood (2005b) and Khairoutdinov and Kogan (2000) schemes do not differ significantly (p=0.05) from the observation-based radiative calculations, while the Liu and Daum (2004) scheme differs significantly from the observation-based calculation for the downward shortwave but not the downward longwave fluxes. This research has been supported by the Natural Sciences and Engineering Research Council of Canada (Discovery Grants RGPIN-2014-05173 and RGPIN 155649) and the Marine Environmental Observation, Prediction and Response Network (MEOPAR), which is a federally funded Networks of Centres of Excellence (NCE) (EC1-RC-DAL). Peer Reviewed Postprint (published version)