| Summary: | Due to possible aragonite to calcite transformation resulting in alteration in isotopic signatures and a bias in age-dating, aragonite speleothems are often excluded from paleoclimatic archives. However, aragonite stalagmites contain ppm-level uranium content, making them much easier to date, achieving higher age-dating precisions than calcite stalagmites. In this regard, provided aragonite-to-calcite transformation did not occur, aragonite stalagmites are potentially well suited for Holocene climate research, given their climate proxies can be placed into a better constrained chronological framework. In this paper, we present high-precision U/Th dates and O isotopic time series for a 82cm long, continuous growth aragonite stalagmite, LH2, from Lianhua Cave, Hunan Province, China, and discuss East Asian Summer Monsoon (EASM) variability for the last 12.5ka BP (before present). The U/Th-dated δO sequence with a mean 16-year resolution and the growth rate pattern of LH2 show that EASM experienced a strengthening stage, a strong stage and a weakening stage during the last 12.5ka. During the YD (12.5-11.5ka BP), heavy δO values and low growth rate indicate a weak monsoon period. During the Preboreal (from ~11.5 to 10.6ka BP), δO values decreased dramatically (~1.94‰) reflecting abrupt strengthening of the monsoon. From 10.6 to 4.2ka BP, the record is characterized by the lightest δO values and high growth rates, suggesting a strong monsoon period. The summer monsoon weakened substantially after 4.2ka BP, as inferred from gradually increasing δO values and decreasing growth rate. Overall, the intensity of the EASM is regulated by summer insolation at 30°N during the last 12.5ka. Although oxygen isotope fractionation is different between aragonite-HO and calcite-HO because of Rayleigh Fractionation Law, the overall temporal pattern of δO values from aragonite stalagmite LH2 is concordant with other high-resolution Holocene calcite stalagmite records from South China. The comparison among these records shows that the Holocene Optimum was synchronous across Asian continental region influenced by the EASM and Indian Summer Monsoon (ISM), lasting from ~10.6 to 4.2ka BP, as reflected by consistently lighter δO values among all these records regardless of their latitudinal difference. These records do not support previously reported asynchronism between EASM and ISM. In details, the long-term δO trend in LH2 is punctuated by a number of centennial fluctuations. For instance, two weak monsoon events occurred at 9232±57yr BP and 8137±21yr BP, correlating in time with cooling events in Greenland ice cores. The latest weak monsoon event centered at 302±8yr BP which is related to the Little Ice Age (LIA). In addition, the monsoon intensity derived from our record also shows a strong connection with latitudinal migration of the Inter-Tropical Convergence Zone (ITCZ) as recorded in the Cariaco Basin sediments. Spectral analysis of δO values shows that significant peaks match with solar periodicities of 208yr (de Vries cycle), 86yr (Gleissberg cycle) or related to δC production suggesting shorter-term monsoon variations are forced by solar radiation. Overall, our study suggests that the δO record in the aragonite stalagmite is highly consistent with those derived from calcite stalagmites, suggesting that aragonite stalagmites are suitable for palaeoclimate reconstruction, especially for the Holocene period, as aragonite-calcite transformation has not occurred.
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