Ozone trends at northern mid- and high latitudes – a European perspective

The EU CANDIDOZ project investigated the chemical and dynamical influences on decadal ozone trends focusing on the Northern Hemisphere. High quality long-term ozone data sets, satellite-based as well as ground-based, and the long-term meteorological reanalyses from ECMWF and NCEP are used together w...

Full description

Bibliographic Details
Main Authors: Harris, Neil R. P., Kyrö, E., Staehelin, J., Brunner, D., Andersen, S.-B., Godin-Beekmann, Sophie, Dhomse, S., Hadjinicolaou, P., Hansen, G., Isaksen, I., Jrrar, A., Karpetchko, A., Kivi, R., Knudsen, B., Krizan, P., Lastovicka, J., Maeder, J., Orsolini, Y., Pyle, J.A., Rex, M., Vanicek, K., Weber, M., Wohltmann, I., Zanis, P., Zerefos, C.
Other Authors: Centre for Atmospheric Science Cambridge, UK, University of Cambridge UK (CAM), European Ozone Research Coordinating Unit Cambridge (EORCU), Arctic Research Centre of Finnish Meteorological Institute, Finnish Meteorological Institute (FMI), Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology Zürich (ETH Zürich), EMPA, Swiss Federal Laboratories for Materials Testing and Research, Danish Meteorological Institute (DMI), Service d'aéronomie (SA), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), University of Bremen, National and Kapodistrian University of Athens (NKUA), Frederick Institute of Technology, Norwegian Institute for Air Research (NILU), University of Oslo (UiO), Institute of Atmospheric Physics Prague (IAP), Czech Academy of Sciences Prague (CAS), Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung = Alfred Wegener Institute for Polar and Marine Research = Institut Alfred-Wegener pour la recherche polaire et marine (AWI), Helmholtz-Gemeinschaft = Helmholtz Association, Czech Hydrometeorological Institute (CHMI), Department of Meteorology and Climatology Thessaloniki, Aristotle University of Thessaloniki
Format: Article in Journal/Newspaper
Language:English
Published: HAL CCSD 2008
Subjects:
Online Access:https://hal.science/hal-00283606
https://hal.science/hal-00283606/document
https://hal.science/hal-00283606/file/angeo-26-1207-2008.pdf
Description
Summary:The EU CANDIDOZ project investigated the chemical and dynamical influences on decadal ozone trends focusing on the Northern Hemisphere. High quality long-term ozone data sets, satellite-based as well as ground-based, and the long-term meteorological reanalyses from ECMWF and NCEP are used together with advanced multiple regression models and atmospheric models to assess the relative roles of chemistry and transport in stratospheric ozone changes. This overall synthesis of the individual analyses in CANDIDOZ shows clearly one common feature in the NH mid latitudes and in the Arctic: an almost monotonic negative trend from the late 1970s to the mid 1990s followed by an increase. In most trend studies, the Equivalent Effective Stratospheric Chlorine (EESC) which peaked in 1997 as a consequence of the Montreal Protocol was observed to describe ozone loss better than a simple linear trend. Furthermore, all individual analyses point to changes in dynamical drivers, such as the residual circulation (responsible for the meridional transport of ozone into middle and high latitudes) playing a key role in the observed turnaround. The changes in ozone transport are associated with variations in polar chemical ozone loss via heterogeneous ozone chemistry on PSCs (polar stratospheric clouds). Synoptic scale processes as represented by the new equivalent latitude proxy, by conventional tropopause altitude or by 250 hPa geopotential height have also been successfully linked to the recent ozone increases in the lowermost stratosphere. These show significant regional variation with a large impact over Europe and seem to be linked to changes in tropospheric climate patterns such as the North Atlantic Oscillation. Some influence in recent ozone increases was also attributed to the rise in solar cycle number 23. Changes from the late 1970s to the mid 1990s were found in a number of characteristics of the Arctic vortex. However, only one trend was found when more recent years are also considered, namely the tendency for cold winters ...