Atmospheric methane over Siberia: measurements from the 2014 YAK-AEROSIB aircraft campaign

International audience The YAK-AEROSIB program collects high-precision in-situ measurements of the vertical distribution of CO2, CH4, CO, O3, black carbon and ultrafine particles distribution in the Siberian troposphere, as well as other parameters including aerosol lidar profiles, on a pan-Siberian...

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Main Authors: Paris, Jean-Daniel, Pisso, Ignacio, Ancellet, Gérard, Law, Kathy S., Arshinov, Mikhail Yu., Belan, Boris D., Nédélec, Philippe, Lund Myhre, Cathrine
Other Authors: Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA), Norwegian Institute for Air Research (NILU), TROPO - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), V.E. Zuev Institute of Atmospheric Optics (IAO), Siberian Branch of the Russian Academy of Sciences (SB RAS), Laboratoire d'aérologie (LAERO), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS)
Format: Conference Object
Language:English
Published: HAL CCSD 2017
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Online Access:https://insu.hal.science/insu-01666108
Description
Summary:International audience The YAK-AEROSIB program collects high-precision in-situ measurements of the vertical distribution of CO2, CH4, CO, O3, black carbon and ultrafine particles distribution in the Siberian troposphere, as well as other parameters including aerosol lidar profiles, on a pan-Siberian aircraft transect. Recent efforts aim at better understanding the respective role of CH4 emission processes in driving its large scale atmospheric variability over the region. The October 2014 YAK-AEROSIB/MOCA campaign from Novosibirsk to Salekhard and over the Kara sea and the Yamal peninsula sampled air masses affected by local, regional and remote pollution. We analyse the contribution of local anthropogenic sources to measured CH4 enhancements, in relation to atmospheric mixing and transport conditions. Our analysis also attempts to detect CH4 signal from sources of methane in the Siberian shelf and the Arctic ocean during low level flight legs over the Kara sea using the airborne measurements and a Lagrangian model coupled to potential CH4 hydrate and geological sources. The measured CH4 concentrations do not contradict a potential source upstream of our measurements, but the interpretation is challenging due to a very low CH4 signal. The challenging question of the methane budget and its evolution in Siberia leads to a need for new approaches. A new generation of airborne measurements, more flexible, is now needed.