Multidecadal trends in aerosol radiative forcing over the Arctic:Contribution of changes in anthropogenic aerosol to Arctic warming since 1980

Arctic observations show large decreases in the concentrations of sulfate and black carbon (BC) aerosols since the early 1980s. These near-term climate-forcing pollutants perturb the radiative balance of the atmosphere and may have played an important role in recent Arctic warming. We use the GEOS-C...

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Bibliographic Details
Published in:Journal of Geophysical Research: Atmospheres
Main Authors: Breider, Thomas J., Mickley, Loretta J., Jacob, Daniel J., Ge, Cui, Wang, Jun, Sulprizio, Melissa Payer, Croft, Betty, Ridley, David A., McConnell, Joseph R., Sharma, Sangeeta, Husain, Liaquat, Dutkiewicz, Vincent A., Eleftheriadis, Konstantinos, Skov, Henrik, Hopke, Phillip K.
Format: Article in Journal/Newspaper
Language:English
Published: 2017
Subjects:
Arctic
aerosol
trends
radiative forcing
anthropogenic
aerosol-radiation interactions
BIOMASS BURNING EMISSIONS
LONG-TERM TRENDS
BLACK CARBON
CLIMATE RESPONSE
INTERANNUAL VARIABILITY
ICE-CORE
TRANSPORT
SULFATE
AIRCRAFT
DISTRIBUTIONS
black carbon
ice core
Online Access:https://pure.au.dk/portal/en/publications/7a828705-df77-4de4-b1fb-c9358dcbadba
https://doi.org/10.1002/2016JD025321
http://www.scopus.com/inward/record.url?scp=85015299463&partnerID=8YFLogxK
Description
Summary:Arctic observations show large decreases in the concentrations of sulfate and black carbon (BC) aerosols since the early 1980s. These near-term climate-forcing pollutants perturb the radiative balance of the atmosphere and may have played an important role in recent Arctic warming. We use the GEOS-Chem global chemical transport model to construct a 3-D representation of Arctic aerosols that is generally consistent with observations and their trends from 1980 to 2010. Observations at Arctic surface sites show significant decreases in sulfate and BC mass concentrations of 2-3% per year. We find that anthropogenic aerosols yield a negative forcing over the Arctic, with an average 2005-2010 Arctic shortwave radiative forcing (RF) of -0.190.05Wm(-2) at the top of atmosphere (TOA). Anthropogenic sulfate in our study yields more strongly negative forcings over the Arctic troposphere in spring (-1.170.10Wm(-2)) than previously reported. From 1980 to 2010, TOA negative RF by Arctic aerosol declined, from -0.670.06Wm(-2) to -0.190.05Wm(-2), yielding a net TOA RF of +0.48 +/- 0.06Wm(-2). The net positive RF is due almost entirely to decreases in anthropogenic sulfate loading over the Arctic. We estimate that 1980-2010 trends in aerosol-radiation interactions over the Arctic and Northern Hemisphere midlatitudes have contributed a net warming at the Arctic surface of +0.27 +/- 0.04K, roughly one quarter of the observed warming. Our study does not consider BC emissions from gas flaring nor the regional climate response to aerosol-cloud interactions or BC deposition on snow.

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