Sources of fine-sized organic matter in North Atlantic Heinrich Layers: δ 13 C and δ 15 N tracers

International audience Organic carbon (OC) and total nitrogen (TN) concentrations and stable isotope ratios (δ 13 C, δ 15 N) of fine (<50 μm) size fractions of deep-sea sediments from the central North Atlantic were employed to identify changes in sources of organic matter over the past 50 ka BP....

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Bibliographic Details
Published in:Geochimica et Cosmochimica Acta
Main Authors: Huon, Sylvain, Grousset, Francis E., Burdloff, Didier, Bardoux, Gérard, Mariotti, André
Other Authors: Institut d'écologie et des sciences de l'environnement de Paris (iEES), Institut National de la Recherche Agronomique (INRA)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Université Paris-Est Créteil Val-de-Marne - Paris 12 (UPEC UP12)-Centre National de la Recherche Scientifique (CNRS), Environnements et Paléoenvironnements OCéaniques (EPOC), Observatoire aquitain des sciences de l'univers (OASU), Université Sciences et Technologies - Bordeaux 1 (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Sciences et Technologies - Bordeaux 1 (UB)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-École Pratique des Hautes Études (EPHE), Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)
Format: Article in Journal/Newspaper
Language:English
Published: HAL CCSD 2002
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Online Access:https://insu.hal.science/insu-03619006
https://doi.org/10.1016/S0016-7037(01)00776-1
Description
Summary:International audience Organic carbon (OC) and total nitrogen (TN) concentrations and stable isotope ratios (δ 13 C, δ 15 N) of fine (<50 μm) size fractions of deep-sea sediments from the central North Atlantic were employed to identify changes in sources of organic matter over the past 50 ka BP. Ambient glacial sediments are characterised by values that reflect mixtures of marine and terrestrial inputs (averages ± 1σ: OC/TN = 7.6 ± 0.8; δ 13 C = -22.8 ± 1.0‰; δ 15 N = 5.5 ± 0.6‰). δ 13 C, OC, and TN concentrations shift to higher values during the Holocene, indicating a gradual decrease of fine terrigenous supply to the North Atlantic. The unchanged δ 15 N record between last glacial and Holocene stages indicates that the central North Atlantic region remained oligotrophic at least during the past 50 ka BP, but additional studies are required to support this result in terms of nitrogen oceanic budget. During the phases of enhanced ice-rafted detrital supply corresponding to prominent Heinrich events (HL 1 , HL 2 , HL 4 , and HL 5 ), fine-sized sedimentary organic matter has lower OC and TN concentrations, contrasting sharply with those of ambient glacial sediments. Lower δ 13 C (down to -28‰) and δ 15 N (down to 1.6‰) values and high OC:TN ratios (up to 14.7 ± 1.1) are found for HL 1 , HL 2 , and with lesser extent for HL 4 . These values reflect enhanced detrital supply originating from poorly differentiated soil horizons that characterise periglacial climate conditions and from organic matter-bearing rock sources of the underlying geological basement. During HL 5 , only the δ 13 C offset records the input of fine size ice-rafted organic matter. Gradually changing soil development conditions during the time interval covering HL 5 to HL 1 (marine isotope stages 5 to 2), as well as varying erosion levels, have been hypothesized on the basis of constant δ 13 C, increasing OC/TN and decreasing δ 15 N values.