The global sources of nitrous oxide

We use atmospheric and ice core data on the concentrations of nitrous oxide to estimate that the present global anthropogenic emissions are 7±1 tg/yr. If the atmospheric lifetime of N2O is a hundred years or more, this estimate is virtually independent of the actual lifetime. The natural sources are...

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Bibliographic Details
Published in:Journal of Geophysical Research
Main Authors: Khalil, M. A. K., Rasmussen, R. A.
Format: Article in Journal/Newspaper
Language:English
Published: AGU (American Geophysical Union) 1992
Subjects:
Online Access:https://oceanrep.geomar.de/id/eprint/29100/
https://oceanrep.geomar.de/id/eprint/29100/1/Khalil.pdf
https://doi.org/10.1029/92JD01222
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Summary:We use atmospheric and ice core data on the concentrations of nitrous oxide to estimate that the present global anthropogenic emissions are 7±1 tg/yr. If the atmospheric lifetime of N2O is a hundred years or more, this estimate is virtually independent of the actual lifetime. The natural sources are estimated to be about 15 tg/yr. We also find that nitrous oxide started increasing rapidly only during the last century. The trends over the last decade are extremely variable; over 3-year periods the trends have ranged from 0.5 ± 0.2 parts per billion by volume (ppbv/yr) to 1.2 ± 0.1 ppbv/yr. The average rate of increase is about 0.80 ± 0.02 ppbv/yr or 0.27 ± 0.01 %/yr (1977–1988). There is an indication that N2O may be increasing faster in recent years than during the middle 1970s by about 0.2 ± 0.1 ppbv/yr. It is likely that several small anthropogenic sources may be causing the present trends, all emitting between 0.1 and 1.5 Tg/yr.