Ice-nucleating particle concentration measurements from Ny-Ålesund during the Arctic spring–summer in 2018

• Published in: Atmospheric Chemistry and Physics
• Main Authors: Rinaldi, Matteo, Hiranuma, Naruki, Santachiara, Gianni, Mazzola, Mauro, Mansour, Karam, Paglione, Marco, Rodriguez, Cheyanne A., Traversi, Rita, Becagli, Silvia, Cappelletti, David, Belosi, Franco
• Format: Article in Journal/Newspaper
• Language: English
• Published: Copernicus Publications 2021
• Subjects: article; Verlagsveröffentlichung; Arctic; Ny-Ålesund; Svalbard; Ny Ålesund
• Online Access: https://doi.org/10.5194/acp-21-14725-2021; https://noa.gwlb.de/receive/cop_mods_00058316; https://noa.gwlb.de/servlets/MCRFileNodeServlet/cop_derivate_00057966/acp-21-14725-2021.pdf; https://acp.copernicus.org/articles/21/14725/2021/acp-21-14725-2021.pdf

In this study, we present atmospheric ice-nucleating particle (INP) concentrations from the Gruvebadet (GVB) observatory in Ny-Ålesund (Svalbard). All aerosol particle sampling activities were conducted in April–August 2018. Ambient INP concentrations (nINP) were measured for aerosol particles collected on filter samples by means of two offline instruments: the Dynamic Filter Processing Chamber (DFPC) and the West Texas Cryogenic Refrigerator Applied to Freezing Test system (WT-CRAFT) to assess condensation and immersion freezing, respectively. DFPC measured nINPs for a set of filters collected through two size-segregated inlets: one for transmitting particulate matter of less than 1 µm (PM1), the other for particles with an aerodynamic diameter of less than 10 µm aerodynamic diameter (PM10). Overall, nINP PM10 measured by DFPC at a water saturation ratio of 1.02 ranged from 3 to 185 m−3 at temperatures (Ts) of −15 to −22 ∘C. On average, the super-micrometer INP (nINP PM10-nINP PM1) accounted for approximately 20 %–30 % of nINP PM10 in spring, increasing in summer to 45 % at −22 ∘C and 65 % at −15 ∘C. This increase in super-micrometer INP fraction towards summer suggests that super-micrometer aerosol particles play an important role as the source of INPs in the Arctic. For the same T range, WT-CRAFT measured 1 to 199 m−3. Although the two nINP datasets were in general agreement, a notable nINP offset was observed, particularly at −15 ∘C. Interestingly, the results of both DFPC and WT-CRAFT measurements did not show a sharp increase in nINP from spring to summer. While an increase was observed in a subset of our data (WT-CRAFT, between −18 and −21 ∘C), the spring-to-summer nINP enhancement ratios never exceeded a factor of 3. More evident seasonal variability was found, however, in our activated fraction (AF) data, calculated by scaling the measured nINP to the total aerosol particle concentration. In 2018, AF increased from spring to summer. This seasonal AF trend corresponds to the overall decrease in aerosol ...