Coalescence scavenging drives droplet number concentration in Southern Ocean low clouds

Cloud droplet number concentration (N-d) is a key microphysical property that is largely controlled by the balance between sources and sinks of aerosols that serve as cloud condensation nuclei (CCN). Despite being a key sink of CCN, the impact of coalescence scavenging on Southern Ocean (SO) cloud i...

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Bibliographic Details
Published in:Geophysical Research Letters
Other Authors: Kang, L. (author), Marchand, R. T. (author), Wood, R. (author), McCoy, Isabel L. (author)
Format: Article in Journal/Newspaper
Language:English
Published: 2022
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Online Access:https://doi.org/10.1029/2022GL097819
Description
Summary:Cloud droplet number concentration (N-d) is a key microphysical property that is largely controlled by the balance between sources and sinks of aerosols that serve as cloud condensation nuclei (CCN). Despite being a key sink of CCN, the impact of coalescence scavenging on Southern Ocean (SO) cloud is poorly known. We apply a simple source-and-sink budget model based on parameterizations to austral summer aircraft observations to test model behavior and examine the relative influence of processes that determine N-d in SO stratocumulus clouds. The model predicts N-d with little bias and a correlation coefficient of similar to 0.7 compared with observations. Coalescence scavenging is found to be an important sink of CCN in both liquid and mixed-phase precipitating stratocumulus and reduces the predicted N-d by as much as 90% depending on the precipitation rate. The free tropospheric aerosol source controls N-d more strongly than the surface aerosol source during austral summer. NA18NWS4620043B