| Summary: | 2020 Spring. Includes bibliographical references. The limited anthropogenic and terrestrial aerosol sources impacting the Southern Ocean (SO) make it a unique site to study the production of primary sea spray aerosols (SSA) and their role in modifying cloud properties. Previous observations of low ice nucleating particle (INP) concentrations and recent modeling work support the idea that the SO INP population is dominated by SSA. These marine INPs are hypothesized to strongly influence the lifetime, formation, and optical properties of the supercooled and mixed phase clouds that are common in the region, though direct observational evidence for this is lacking. This study focuses on improving our understanding of INP emissions in the marine boundary layer over the SO, with applicability to other ocean regions, and to provide in situ measurements with which to validate and improve INP parameterizations in global and cloud resolving models. Measurements of INPs and aerosols in the marine boundary layer were made during the Clouds, Aerosols, Precipitation Radiation and atmospherIc Composition Over the southeRN ocean 2 (CAPRICORN-2) study on the R/V Investigator during Jan. - March 2018. An initial focus of this thesis was on increasing speed and reproducibility of processing online INP measurements, as well as improving the determination of statistical significance and uncertainty bounds. Different approaches to parameterizing INPs in models are explored for SO aerosols, including the use of aerosol surface area and number concentrations. With an eye towards augmenting global datasets of INPs, a comparison of particle surface area measurements from four different techniques is presented, for use in developing and testing INP parameterizations for different sources and atmospheric conditions. Surface area concentrations derived from Wideband Integrated Bioaerosol Sensor (WIBS) and nephelometer observations are strongly correlated with direct particle size distribution measurements, and can be used in their ...
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