Does Cosmic-Ray-Induced Heterogeneous Chemistry Influence Stratospheric Polar Ozone Loss ?

Cosmic-ray (CR) -induced heterogeneous reactions of halogenated species have been suggested to play the dominant role in causing the Antarctic ozone hole. However, measurements of total ozone in Antarctica do not show a compact and significant correlation with CR activity. Further, a substantial CR-...

Full description

Bibliographic Details
Published in:Physical Review Letters
Main Authors: Müller, R., Grooß, J.-U.
Format: Article in Journal/Newspaper
Language:English
Published: APS 2009
Subjects:
J
Online Access:https://juser.fz-juelich.de/record/4948
https://juser.fz-juelich.de/search?p=id:%22PreJuSER-4948%22
Description
Summary:Cosmic-ray (CR) -induced heterogeneous reactions of halogenated species have been suggested to play the dominant role in causing the Antarctic ozone hole. However, measurements of total ozone in Antarctica do not show a compact and significant correlation with CR activity. Further, a substantial CR-induced heterogeneous loss of chlorofluorocarbons is incompatible with multiyear satellite observations of N2O and CFC-12. Thus, CR-induced heterogeneous reactions cannot be considered as an alternative mechanism causing the Antarctic ozone hole.