Airmass Analysis of Size-Resolved Black Carbon Particles Observed in the Arctic Based on Cluster Analysis

Here we apply new analysis methods and approaches to existing long-term measurement series that provide additional insights into the atmospheric processes that control black carbon (BC) in the Arctic. Based on clustering size distribution data from Zeppelin Observatory for the years 2002–2010, obser...

Full description

Bibliographic Details
Published in:Atmosphere
Main Authors: Roxana S. Cremer, Peter Tunved, Johan Ström
Format: Article in Journal/Newspaper
Language:English
Published: MDPI AG 2022
Subjects:
Online Access:https://doi.org/10.3390/atmos13050648
https://doaj.org/article/c82148a0c84b457da28e150948296fc0
Description
Summary:Here we apply new analysis methods and approaches to existing long-term measurement series that provide additional insights into the atmospheric processes that control black carbon (BC) in the Arctic. Based on clustering size distribution data from Zeppelin Observatory for the years 2002–2010, observations classified as ‘Polluted’ were further investigated based on BC properties. The data were split into two subgroups, and while the microphysical and chemical fingerprints of the two subgroups are very similar, they show larger differences in BC concentration and correlation with the particle size distribution. Therefore, a source–receptor analysis was performed with HYSPLIT 10-days backward trajectories for both subsets. We demonstrate that within this ‘Polluted’ category, the airmasses that contributed to the largest BC signal at the Zeppelin station are not necessarily associated with traditional transport pathways from Eurasia. Instead, the strongest signal is from a region east of the Ural Mountains across the continent to the Kamchatka Peninsula.