Measurement report: The chemical composition of and temporal variability in aerosol particles at Tuktoyaktuk, Canada, during the Year of Polar Prediction Second Special Observing Period

The chemical composition, sources, and concentrations of aerosol particles vary on a seasonal basis in the Arctic. While existing research has focused on understanding the occurrence of aerosol particles during the Arctic winter and spring, less is known of their occurrence during the Arctic summer....

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Bibliographic Details
Published in:Atmospheric Chemistry and Physics
Main Authors: J. MacInnis, J. P. Chaubey, C. Weagle, D. Atkinson, R. Y.-W. Chang
Format: Article in Journal/Newspaper
Language:English
Published: Copernicus Publications 2021
Subjects:
Online Access:https://doi.org/10.5194/acp-21-14199-2021
https://doaj.org/article/bf00ce98b2c64c5b881457dd4d1dfdbd
Description
Summary:The chemical composition, sources, and concentrations of aerosol particles vary on a seasonal basis in the Arctic. While existing research has focused on understanding the occurrence of aerosol particles during the Arctic winter and spring, less is known of their occurrence during the Arctic summer. In this study, atmospheric aerosol particle chemical composition and concentration were determined during July–September 2018 at Tuktoyaktuk, NT, Canada (69.4 ∘ N, 133.0 ∘ W), to coincide with the Year of Polar Prediction's Second Special Observing Period in the Arctic. The chemical composition of fine (PM 2.5 ) and coarse (PM 10–2.5 ) aerosol filter samples suggests the ocean, mineral and/or road dust, and combustion were sources of the sampled aerosol particles. Mass concentrations of PM 2 and PM 10 , estimated from optical particle counter measurements, remained within a similar range during the study. However, elevated mass concentrations coincided with a festival in the community of Tuktoyaktuk, suggesting local human activity was an important source of aerosol particles. Mass concentrations of PM 2 , which promote negative health effects in humans, were significantly lower at Tuktoyaktuk than the national air quality standard recommended by the government of Canada. These measurements provide an important baseline to compare with future measurements associated with the assessment of aerosol chemistry and air quality in the Arctic.