A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy

Cavity ring-down spectroscopy (CRDS) has allowed for increasingly widespread, in situ observations of trace gases, including the stable isotopic composition of water vapor. However, gathering observations in harsh environments still poses challenges, particularly in regard to observing the small-sca...

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Published in:Atmospheric Measurement Techniques
Main Authors: A. W. Seidl, H. Sodemann, H. C. Steen-Larsen
Format: Article in Journal/Newspaper
Language:English
Published: Copernicus Publications 2023
Subjects:
Online Access:https://doi.org/10.5194/amt-16-769-2023
https://doaj.org/article/ab689607426e4eb9bc5a72bcbe5fe5dd
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author A. W. Seidl
H. Sodemann
H. C. Steen-Larsen
author_facet A. W. Seidl
H. Sodemann
H. C. Steen-Larsen
author_sort A. W. Seidl
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description Cavity ring-down spectroscopy (CRDS) has allowed for increasingly widespread, in situ observations of trace gases, including the stable isotopic composition of water vapor. However, gathering observations in harsh environments still poses challenges, particularly in regard to observing the small-scale exchanges taking place between the surface and atmosphere. It is especially important to resolve the vertical structure of these processes. We have designed the ISE-CUBE system as a modular CRDS deployment system for profiling stable water isotopes in the surface layer, specifically the lowermost 2 m above the surface. We tested the system during a 2-week field campaign during February–March 2020 in Ny-Ålesund, Svalbard, Norway, with ambient temperatures down to −30 ∘ C. The system functioned suitably throughout the campaign, with field periods exhibiting only a marginal increase in isotopic measurement uncertainty (30 %) as compared to optimal laboratory operation. Over the 2 m profiling range, we have been able to measure and resolve gradients on the temporal and spatial scales needed in an Arctic environment.
format Article in Journal/Newspaper
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Ny Ålesund
Ny-Ålesund
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geographic Arctic
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spelling ftdoajarticles:oai:doaj.org/article:ab689607426e4eb9bc5a72bcbe5fe5dd 2025-01-16T20:37:37+00:00 A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy A. W. Seidl H. Sodemann H. C. Steen-Larsen 2023-02-01T00:00:00Z https://doi.org/10.5194/amt-16-769-2023 https://doaj.org/article/ab689607426e4eb9bc5a72bcbe5fe5dd EN eng Copernicus Publications https://amt.copernicus.org/articles/16/769/2023/amt-16-769-2023.pdf https://doaj.org/toc/1867-1381 https://doaj.org/toc/1867-8548 doi:10.5194/amt-16-769-2023 1867-1381 1867-8548 https://doaj.org/article/ab689607426e4eb9bc5a72bcbe5fe5dd Atmospheric Measurement Techniques, Vol 16, Pp 769-790 (2023) Environmental engineering TA170-171 Earthwork. Foundations TA715-787 article 2023 ftdoajarticles https://doi.org/10.5194/amt-16-769-2023 2023-02-12T01:29:09Z Cavity ring-down spectroscopy (CRDS) has allowed for increasingly widespread, in situ observations of trace gases, including the stable isotopic composition of water vapor. However, gathering observations in harsh environments still poses challenges, particularly in regard to observing the small-scale exchanges taking place between the surface and atmosphere. It is especially important to resolve the vertical structure of these processes. We have designed the ISE-CUBE system as a modular CRDS deployment system for profiling stable water isotopes in the surface layer, specifically the lowermost 2 m above the surface. We tested the system during a 2-week field campaign during February–March 2020 in Ny-Ålesund, Svalbard, Norway, with ambient temperatures down to −30 ∘ C. The system functioned suitably throughout the campaign, with field periods exhibiting only a marginal increase in isotopic measurement uncertainty (30 %) as compared to optimal laboratory operation. Over the 2 m profiling range, we have been able to measure and resolve gradients on the temporal and spatial scales needed in an Arctic environment. Article in Journal/Newspaper Arctic Ny Ålesund Ny-Ålesund Svalbard Directory of Open Access Journals: DOAJ Articles Arctic Norway Ny-Ålesund Svalbard Atmospheric Measurement Techniques 16 3 769 790
spellingShingle Environmental engineering
TA170-171
Earthwork. Foundations
TA715-787
A. W. Seidl
H. Sodemann
H. C. Steen-Larsen
A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_full A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_fullStr A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_full_unstemmed A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_short A modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
title_sort modular field system for near-surface, vertical profiling of the atmospheric composition in harsh environments using cavity ring-down spectroscopy
topic Environmental engineering
TA170-171
Earthwork. Foundations
TA715-787
topic_facet Environmental engineering
TA170-171
Earthwork. Foundations
TA715-787
url https://doi.org/10.5194/amt-16-769-2023
https://doaj.org/article/ab689607426e4eb9bc5a72bcbe5fe5dd