Comparison of the aerosol optical properties and size distribution retrieved by sun photometer with in situ measurements at midlatitude

• Published in: Atmospheric Measurement Techniques
• Main Authors: A. Chauvigné, K. Sellegri, M. Hervo, N. Montoux, P. Freville, P. Goloub
• Format: Article in Journal/Newspaper
• Language: English
• Published: Copernicus Publications 2016
• Subjects: Environmental engineering; TA170-171; Earthwork. Foundations; TA715-787; Aerosol Robotic Network
• Online Access: https://doi.org/10.5194/amt-9-4569-2016; https://doaj.org/article/3604386db3294fdd8479da1e6cee770c

Aerosols influence the Earth radiative budget through scattering and absorption of solar radiation. Several methods are used to investigate aerosol properties and thus quantify their direct and indirect impacts on climate. At the Puy de Dôme station, continuous high-altitude near-surface in situ measurements and low-altitude ground-based remote sensing atmospheric column measurements give the opportunity to compare the aerosol extinction measured with both methods over a 1-year period. To our knowledge, it is the first time that such a comparison is realised with continuous measurements of a high-altitude site during a long-term period. This comparison addresses to which extent near-surface in situ measurements are representative of the whole atmospheric column, the aerosol mixing layer (ML) or the free troposphere (FT). In particular, the impact of multi-aerosol layers events detected using lidar backscatter profiles is analysed. A good correlation between in situ aerosol extinction coefficient and aerosol optical depth (AOD) measured by the Aerosol Robotic Network (AERONET) sun photometer is observed with a correlation coefficient around 0.80, indicating that the in situ measurements station is representative of the overall atmospheric column. After filtering for multilayer cases and correcting for each layer optical contribution (ML and FT), the atmospheric structure seems to be the main factor influencing the comparison between the two measurement techniques. When the site lies in the ML, the in situ extinction represents 45 % of the sun photometer ML extinction while when the site lies within the FT, the in situ extinction is more than 2 times higher than the FT sun photometer extinction. Moreover, the assumption of a decreasing linear vertical aerosol profile in the whole atmosphere has been tested, significantly improving the instrumental agreement. Remote sensing retrievals of the aerosol particle size distributions (PSDs) from the sun photometer observations are then compared to the near-surface in situ ...