Microgram level radiocarbon (14C) determination on carbonaceous particles in ice ...

In climate research the interest on carbonaceous particles has increased over the last years because of their influence on the radiation balance of the earth. Nevertheless, there is a paucity of available data regarding their concentrations and sources in the past. Such data would be important for a...

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Bibliographic Details
Main Authors: Jenk, Theo, Szidat, Sönke, Wacker, L, Saurer, M, Synal, H, Gäggeler, Heinz, Schwikowski, Margit
Format: Text
Language:English
Published: Elsevier 2007
Subjects:
Online Access:https://dx.doi.org/10.7892/boris.22423
http://boris.unibe.ch/22423/
Description
Summary:In climate research the interest on carbonaceous particles has increased over the last years because of their influence on the radiation balance of the earth. Nevertheless, there is a paucity of available data regarding their concentrations and sources in the past. Such data would be important for a better understanding of their effects and for estimating their influence on future climate. Here, a technique is described to extract carbonaceous particles from ice core samples with subsequent separation of the two main constituents into organic carbon (OC) and elemental carbon (EC) for analysis of their concentrations in the past. This is combined with further analysis of OC and EC 14C/12C ratios by accelerator mass spectrometry (AMS), what can be used for source apportionment studies of past emissions. We further present how 14C analysis of the OC fraction could be used in the future to date any ice core extracted from a high-elevation glacier. Described sample preparation steps to final analysis include the ...