How well are aerosol-cloud interactions represented in climate models? - Part 1: Understanding the sulfate aerosol production from the 2014-15 Holuhraun eruption ...
For over 6 months, the 2014-2015 effusive eruption at Holuhraun, Iceland, injected considerable amounts of sulfur dioxide (SO2) into the lower troposphere with a daily rate of up to one-third of the global emission rate, causing extensive air pollution across Europe. The large injection of SO2, whic...
Main Authors: | , , , , , , , , , , , , , |
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Format: | Article in Journal/Newspaper |
Language: | English |
Published: |
ETH Zurich
2024
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Subjects: | |
Online Access: | https://dx.doi.org/10.3929/ethz-b-000663171 http://hdl.handle.net/20.500.11850/663171 |
Summary: | For over 6 months, the 2014-2015 effusive eruption at Holuhraun, Iceland, injected considerable amounts of sulfur dioxide (SO2) into the lower troposphere with a daily rate of up to one-third of the global emission rate, causing extensive air pollution across Europe. The large injection of SO2, which oxidises to form sulfate aerosol (SO42-), provides a natural experiment offering an ideal opportunity to scrutinise state-of-the-art general circulation models' (GCMs) representation of aerosol-cloud interactions (ACIs). Here we present Part 1 of a two-part model inter-comparison using the Holuhraun eruption as a framework to analyse ACIs. We use SO2 retrievals from the Infrared Atmospheric Sounding Interferometer (IASI) instrument and ground-based measurements of SO2 and SO42- mass concentrations across Europe, in conjunction with a trajectory analysis using the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model, to assess the spatial and chemical evolution of the volcanic plume as ... : Atmospheric Chemistry and Physics, 24 (3) ... |
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