Molecular and radiocarbon constraints on sources and degradation of terrestrial organic carbon along the Kolyma paleoriver transect, East Siberian Sea ...

Climate warming in northeastern Siberia may induce thaw-mobilization of the organic carbon (OC) now held in permafrost. This study investigated the composition of terrestrial OC exported to Arctic coastal waters to both obtain a natural integration of terrestrial permafrost OC release and to further...

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Bibliographic Details
Main Authors: Vonk, Jorien, Sánchez-García, Laura, Semiletov, Igor P., Dudarev, Oleg V., Eglinton, Timothy I., Andersson, August, Gustafsson, Örjan
Format: Article in Journal/Newspaper
Language:English
Published: ETH Zurich 2010
Subjects:
Online Access:https://dx.doi.org/10.3929/ethz-b-000028788
http://hdl.handle.net/20.500.11850/28788
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Summary:Climate warming in northeastern Siberia may induce thaw-mobilization of the organic carbon (OC) now held in permafrost. This study investigated the composition of terrestrial OC exported to Arctic coastal waters to both obtain a natural integration of terrestrial permafrost OC release and to further understand the fate of released carbon in the extensive Siberian Shelf Seas. Application of a variety of elemental, molecular and isotopic (δ13C and Δ14C) analyses of both surface water suspended particulate matter and underlying surface sediments along a 500 km transect from Kolyma River mouth to the mid-shelf of the East Siberian Sea yielded information on the sources, degradation status and transport processes of thaw-mobilized soil OC. A three end-member dual-carbon-isotopic mixing model was applied to deduce the relative contributions from riverine, coastal erosion and marine sources. The mixing model was solved numerically using Monte Carlo simulations to obtain a fair representation of the uncertainties of ... : Biogeosciences, 7 (10) ...