Sea ice as a source of sea salt aerosol to Greenland ice cores: a model-based study ...

Abstract. Growing evidence suggests that the sea ice surface is an important source of sea salt aerosol and this has significant implications for polar climate and atmospheric chemistry. It also offers the opportunity to use ice core sea salt records as proxies for past sea ice extent. To explore th...

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Bibliographic Details
Main Authors: Rhodes, Rachael H, Yang, Xin, Wolff, Eric W, McConnell, Joseph R, Frey, Markus M
Format: Article in Journal/Newspaper
Language:English
Published: Copernicus Publications 2017
Subjects:
Online Access:https://dx.doi.org/10.17863/cam.27080
https://www.repository.cam.ac.uk/handle/1810/279709
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Summary:Abstract. Growing evidence suggests that the sea ice surface is an important source of sea salt aerosol and this has significant implications for polar climate and atmospheric chemistry. It also offers the opportunity to use ice core sea salt records as proxies for past sea ice extent. To explore this possibility in the Arctic region, we use a chemical transport model to track the emission, transport and deposition of sea salt from both the open ocean and the sea ice, allowing us to assess the relative importance of each. Our results confirm the importance of sea ice sea salt (SISS) to the winter Arctic aerosol burden. For the first time, we explicitly simulate the sea salt concentrations of Greenland snow and find they match high resolution Greenland ice core records to within a factor of two. Our simulations suggest that SISS contributes to the winter maxima in sea salt characteristic of ice cores across Greenland. A north-south gradient in the contribution of SISS relative to open ocean sea salt (OOSS) ...