Trends of anthropogenic CO2 storage in North Atlantic water masses
A high-quality inorganic carbon system database, spanning over three decades (1981–2006) and comprising of 13 cruises, has allowed the applying of the ϕ C° T method and coming up with estimates of the anthropogenic CO 2 ( C ant ) stored in the main water masses of the North Atlantic. In the studied...
| Published in: | Biogeosciences |
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| Main Authors: | , , , , , |
| Format: | Text |
| Language: | English |
| Published: |
2018
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| Subjects: | |
| Online Access: | https://doi.org/10.5194/bg-7-1789-2010 https://www.biogeosciences.net/7/1789/2010/ |
| Summary: | A high-quality inorganic carbon system database, spanning over three decades (1981–2006) and comprising of 13 cruises, has allowed the applying of the ϕ C° T method and coming up with estimates of the anthropogenic CO 2 ( C ant ) stored in the main water masses of the North Atlantic. In the studied region, strong convective processes convey surface properties, like C ant , into deeper ocean layers and grants this region an added oceanographic interest from the point of view of air-sea CO 2 exchanges. Generally, a tendency for decreasing C ant storage rates towards the deep layers has been observed. In the Iberian Basin, the North Atlantic Deep Water has low C ant concentrations and negligible storage rates, while the North Atlantic Central Water in the upper layers shows the largest C ant values and the largest annual increase of its average concentration (1.13 ± 0.14 μmol kg −1 yr −1 ). This unmatched rate of change in the C ant concentration of the warm upper limb of the Meridional Overturning Circulation decreases towards the Irminger basin (0.68 ± 0.06 μmol kg −1 yr −1 ) due to the lowering of the buffering capacity. The mid and deep waters in the Irminger Sea show rather similar C ant concentration rates of increase (between 0.33 and 0.45 μmol kg −1 yr −1 ), whereas in the Iceland basin these layers seem to have been less affected by C ant . Overall, the C ant storage rates in the North Atlantic subpolar gyre during the first half of the 1990s, when a high North Atlantic Oscillation (NAO) phase was dominant, are ~48% higher than during the 1997–2006 low NAO phase that followed. This result suggests that a net decrease in the strength of the North Atlantic sink of atmospheric CO 2 has taken place during the present decade. The changes in deep-water ventilation are the main driving processes causing this weakening of the North Atlantic CO 2 sink. |
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