Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs)
the Arctic stratosphere by in-situ measurements onboard the high-altitude research aircraft Geophysica. Low number densities (∼10−4 cm−3) of small nitric acid (HNO3) containing particles (d<6 µm) were observed at altitudes between 18 and 20 km. Provided the temperatures remain below the NAT equil...
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ftciteseerx:oai:CiteSeerX.psu:10.1.1.404.8157 2023-05-15T15:02:54+02:00 Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs) C. Voigt H. Schlager B. P. Luo A. Dörnbrack A. Roiger P. Stock J. Curtius H. Vössing S. Borrmann S. Davies P. Konopka C. Schiller G. Shur T. Peter The Pennsylvania State University CiteSeerX Archives 2005 application/pdf http://citeseerx.ist.psu.edu/viewdoc/summary?doi=10.1.1.404.8157 http://hal.archives-ouvertes.fr/docs/00/29/56/66/PDF/acp-5-1371-2005.pdf en eng http://citeseerx.ist.psu.edu/viewdoc/summary?doi=10.1.1.404.8157 http://hal.archives-ouvertes.fr/docs/00/29/56/66/PDF/acp-5-1371-2005.pdf Metadata may be used without restrictions as long as the oai identifier remains attached to it. http://hal.archives-ouvertes.fr/docs/00/29/56/66/PDF/acp-5-1371-2005.pdf text 2005 ftciteseerx 2016-01-08T03:00:00Z the Arctic stratosphere by in-situ measurements onboard the high-altitude research aircraft Geophysica. Low number densities (∼10−4 cm−3) of small nitric acid (HNO3) containing particles (d<6 µm) were observed at altitudes between 18 and 20 km. Provided the temperatures remain below the NAT equilibrium temperature TNAT, these NAT particles have the potential to grow further and to remove HNO3 from the stratosphere, thereby enhancing polar ozone loss. Interestingly, the NAT particles formed in less than a day at temperatures just slightly below TNAT (T>TNAT−3.1 K). This unique measurement of PSC formation at extremely low NAT saturation ratios (SNAT�10) constrains current NAT nucleation theories. We suggest, that the NAT particles have formed heterogeneously, but for certain not on ice. Conversely, meteoritic particles may be favorable candidates for triggering NAT nucleation at the observed low number densities. 1 Text Arctic Unknown Arctic |
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ftciteseerx |
language |
English |
description |
the Arctic stratosphere by in-situ measurements onboard the high-altitude research aircraft Geophysica. Low number densities (∼10−4 cm−3) of small nitric acid (HNO3) containing particles (d<6 µm) were observed at altitudes between 18 and 20 km. Provided the temperatures remain below the NAT equilibrium temperature TNAT, these NAT particles have the potential to grow further and to remove HNO3 from the stratosphere, thereby enhancing polar ozone loss. Interestingly, the NAT particles formed in less than a day at temperatures just slightly below TNAT (T>TNAT−3.1 K). This unique measurement of PSC formation at extremely low NAT saturation ratios (SNAT�10) constrains current NAT nucleation theories. We suggest, that the NAT particles have formed heterogeneously, but for certain not on ice. Conversely, meteoritic particles may be favorable candidates for triggering NAT nucleation at the observed low number densities. 1 |
author2 |
The Pennsylvania State University CiteSeerX Archives |
format |
Text |
author |
C. Voigt H. Schlager B. P. Luo A. Dörnbrack A. Roiger P. Stock J. Curtius H. Vössing S. Borrmann S. Davies P. Konopka C. Schiller G. Shur T. Peter |
spellingShingle |
C. Voigt H. Schlager B. P. Luo A. Dörnbrack A. Roiger P. Stock J. Curtius H. Vössing S. Borrmann S. Davies P. Konopka C. Schiller G. Shur T. Peter Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs) |
author_facet |
C. Voigt H. Schlager B. P. Luo A. Dörnbrack A. Roiger P. Stock J. Curtius H. Vössing S. Borrmann S. Davies P. Konopka C. Schiller G. Shur T. Peter |
author_sort |
C. Voigt |
title |
Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs) |
title_short |
Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs) |
title_full |
Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs) |
title_fullStr |
Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs) |
title_full_unstemmed |
Atmospheric Chemistry and Physics Nitric Acid Trihydrate (NAT) formation at low NAT supersaturation in Polar Stratospheric Clouds (PSCs) |
title_sort |
atmospheric chemistry and physics nitric acid trihydrate (nat) formation at low nat supersaturation in polar stratospheric clouds (pscs) |
publishDate |
2005 |
url |
http://citeseerx.ist.psu.edu/viewdoc/summary?doi=10.1.1.404.8157 http://hal.archives-ouvertes.fr/docs/00/29/56/66/PDF/acp-5-1371-2005.pdf |
geographic |
Arctic |
geographic_facet |
Arctic |
genre |
Arctic |
genre_facet |
Arctic |
op_source |
http://hal.archives-ouvertes.fr/docs/00/29/56/66/PDF/acp-5-1371-2005.pdf |
op_relation |
http://citeseerx.ist.psu.edu/viewdoc/summary?doi=10.1.1.404.8157 http://hal.archives-ouvertes.fr/docs/00/29/56/66/PDF/acp-5-1371-2005.pdf |
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Metadata may be used without restrictions as long as the oai identifier remains attached to it. |
_version_ |
1766334815438635008 |