© Author(s) 2007. This work is licensed under a Creative Commons License. Atmospheric Chemistry and Physics GEM/POPs: a global 3-D dynamic model for semi-volatile persistent

Abstract. Global transports and budgets of three PCBs were investigated with a 3-D dynamic model for semi-volatile persistent organic pollutants – GEM/POPs. Dominant pathways were identified for PCB transports in the atmosphere with a transport flux peaking below 8 km for gaseous and 14 km for parti...

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Bibliographic Details
Main Authors: P. Huang, S. L. Gong, T. L. Zhao, L. Neary, L. A. Barrie
Other Authors: The Pennsylvania State University CiteSeerX Archives
Format: Text
Language:English
Published: 2007
Subjects:
Online Access:http://citeseerx.ist.psu.edu/viewdoc/summary?doi=10.1.1.404.5058
http://hal.archives-ouvertes.fr/docs/00/29/63/02/PDF/acp-7-4015-2007.pdf
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Summary:Abstract. Global transports and budgets of three PCBs were investigated with a 3-D dynamic model for semi-volatile persistent organic pollutants – GEM/POPs. Dominant pathways were identified for PCB transports in the atmosphere with a transport flux peaking below 8 km for gaseous and 14 km for particulate PCB28, and peaking below 4 km for gaseous and 6 km for particulate PCB180. The inter-continental transports of PCBs in the Northern Hemisphere (NH) are dominated in the zonal direction with their route changes regulated seasonally by the variation of westerly jet. The transport pathways from Europe and North Atlantic contributed the most PCBs to the Arctic. Inter-hemispheric transports of PCBs originated from the regions of Europe, Asia and North America in three different flow-paths, accompanying with easterly jet, Asian monsoon winds and trade winds. PCBs