due to long-range transport of biomass burning emissions

Abstract. Soils and forests in the boreal region of the Northern Hemisphere are recognised as having a large capacity for storing air-borne Persistent Organic Pollutants (POPs), such as the polychlorinated biphenyls (PCBs). Following reductions of primary emissions of various legacy POPs, there is a...

Full description

Bibliographic Details
Main Authors: S. Eckhardt, K. Breivik, S. Manø, A. Stohl
Other Authors: The Pennsylvania State University CiteSeerX Archives
Format: Text
Language:English
Published: 2007
Subjects:
Online Access:http://citeseerx.ist.psu.edu/viewdoc/summary?doi=10.1.1.404.4727
http://hal.archives-ouvertes.fr/docs/00/29/63/23/PDF/acp-7-4527-2007.pdf
Description
Summary:Abstract. Soils and forests in the boreal region of the Northern Hemisphere are recognised as having a large capacity for storing air-borne Persistent Organic Pollutants (POPs), such as the polychlorinated biphenyls (PCBs). Following reductions of primary emissions of various legacy POPs, there is an increasing interest and debate about the relative importance of secondary re-emissions on the atmospheric levels of POPs. In spring of 2006, biomass burning emissions from agricultural fires in Eastern Europe were transported to the Zeppelin station on Svalbard, where record-high levels of many air pollutants were recorded (Stohl et al., 2007). Here we report on the extremely high concentrations of PCBs that were also measured during this period. 21 out of 32 PCB congeners were enhanced by more than two standard deviations above the long-term mean concentrations. In July 2004