Black carbon (BC) in a northern Tibetan mountain: effect of Kuwait fires on glaciers

• Published in: Atmospheric Chemistry and Physics
• Main Authors: Zhou, Jiamao, Tie, Xuexi, Xu, Baiqing, Zhao, Shuyu, Wang, Mo, Li, Guohui, Zhang, Ting, Zhao, Zhuzi, Liu, Suixin, Yang, Song, Chang, Luyu, Cao, Junji
• Format: Report
• Language: English
• Published: COPERNICUS GESELLSCHAFT MBH 2018
• Subjects: ICE CORE; SEASONAL-VARIATIONS; HIMALAYAN GLACIERS; CHEMICAL TRACERS; SPECTRAL ALBEDO; GLOBAL OCEANS; CLIMATE MODEL; SNOW; DEPOSITION; TRANSPORT; Meteorology & Atmospheric Sciences; Indian; Tibetan Mountain; ice core
• Online Access: http://ir.ieecas.cn/handle/361006/7937; https://doi.org/10.5194/acp-18-13673-2018

The black carbon (BC) deposition on the ice core at Muztagh Ata Mountain, northern Tibetan Plateau, was analyzed. Two sets of measurements were used in this study, which included the air samplings of BC particles during 2004-2006 and the ice core drillings of BC deposition during 1986-1994. Two numerical models were used to analyze the measured data. A global chemical transportation model (MOZART-4) was used to analyze the BC transport from the source regions, and a radiative transfer model (SNICAR) was used to study the effect of BC on snow albedo. The results show that during 1991-1992, there was a strong spike in the BC deposition at Muztagh Ata, suggesting that there was an unusual emission in the upward region during this period. This high peak of BC deposition was investigated by using the global chemical transportation model (MOZART-4). The analysis indicated that the emissions from large Kuwait fires at the end of the first Gulf War in 1991 caused this high peak of the BC concentrations and deposition (about 3-4 times higher than other years) at Muztagh Ata Mountain, suggesting that the upward BC emissions had important impacts on this remote site located on the northern Tibetan Plateau. Thus, there is a need to quantitatively estimate the effect of surrounding emissions on the BC concentrations on the northern Tibetan Plateau. In this study, a sensitivity study with four individual BC emission regions (Central Asia, Europe, the Persian Gulf, and South Asia) was conducted by using the MOZART-4 model. The result suggests that during the "normal period" (non-Kuwait fires), the largest effect was due to the Central Asia source (44 %) during the Indian monsoon period, while during the non-monsoon period, the largest effect was due to the South Asia source (34 %). The increase in radiative forcing increase (RFI) due to the deposition of BC on snow was estimated by using the radiative transfer model (SNICAR). The results show that under the fresh snow assumption, the estimated increase in RFI ranged from 0.2 ...