Composition of Ultracarbonaceous Antarctic Micrometeorites (UCAMMs). Comparison with Rosetta/COSIMA Analyses

International audience Introduction: Ultracarbonaceous Antarctic Micrometeorites (UCAMMs) are dominated by a polyaromatic organic matter globally N-enriched showing bulk D enrichments, with heterogeneous distributions of the D/H and 15 N/ 14 N isotopic ratios [1-6]. The abundant organic matter of UC...

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Main Authors: Engrand, Cecile, Dartois, E., Duprat, J., Charon, E., Leroux, H., Le Guillou, C., Bernard, S, Benzerara, Karim, Swaraj, Sufal, Belkhou, Rachid, Delauche, L., Godard, M., Augé, Basile
Other Authors: Centre de Sciences Nucléaires et de Sciences de la Matière (CSNSM), Centre National de la Recherche Scientifique (CNRS)-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3)-Université Paris-Sud - Paris 11 (UP11), Institut d'astrophysique spatiale (IAS), Université Paris-Sud - Paris 11 (UP11)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Centre de Sciences Nucléaires et de Sciences de la Matière (CSNSM AS), Université Paris-Saclay-Univ. Paris-Sud-Institut National de Physique Nucléaire et de Physique des Particules du CNRS (IN2P3), Laboratoire Edifices Nanométriques (LEDNA), Nanosciences et Innovation pour les Matériaux, la Biomédecine et l'Energie (ex SIS2M) (NIMBE UMR 3685), Institut Rayonnement Matière de Saclay (IRAMIS), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Institut Rayonnement Matière de Saclay (IRAMIS), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC), Unité Matériaux et Transformations - UMR 8207 (UMET), Institut de Chimie du CNRS (INC)-Institut National de la Recherche Agronomique (INRA)-Centre National de la Recherche Scientifique (CNRS)-Université de Lille-Ecole Nationale Supérieure de Chimie de Lille (ENSCL), Laboratoire de géologie de l'ENS (LGENS), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Institut de minéralogie, de physique des matériaux et de cosmochimie (IMPMC), Muséum national d'Histoire naturelle (MNHN)-Institut de recherche pour le développement IRD : UR206-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), Synchrotron SOLEIL (SSOLEIL), Centre National de la Recherche Scientifique (CNRS)
Format: Conference Object
Language:English
Published: HAL CCSD 2018
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Online Access:https://hal.archives-ouvertes.fr/hal-02395336
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Summary:International audience Introduction: Ultracarbonaceous Antarctic Micrometeorites (UCAMMs) are dominated by a polyaromatic organic matter globally N-enriched showing bulk D enrichments, with heterogeneous distributions of the D/H and 15 N/ 14 N isotopic ratios [1-6]. The abundant organic matter of UCAMMs contains amorphous and crystalline mineral components [7-9]. This high abundance of organic matter is reminiscent of the CHON particles detected in comet 1P/Halley [10, 11], although the size of CHONs was estimated to be on the micrometer to sub-micrometer size, while UCAMMs from the Concordia collection range in size from ~ 30 µm to ~ 200 µm [12]. They most probably originate from the outer regions of the protoplanetary disk, from the cometary reservoir [1, 3, 4], thus we aim at comparing their composition with that of dust particles from comet 67P/Churyumov-Gerasimenko (hereafter 67P) measured by Ro-setta/COSIMA [13-15]. A recent summary of the general UCAMM characteristics can be found in [12]. Methods: UCAMMs from the Concordia collection were identified by SEM/EDX, and complementary UCAMM fragments were analyzed by synchrotron-based Fourier transform infrared (FTIR) microscopy at SOLEIL/SMIS, electron microprobe analysis (EMPA) at the CAMPARIS facility (Paris), transmission electron microscopy (TEM) at UMET (Lille), STXM-XANES analyses at synchrotron facilities (ALS Berkeley and SOLEIL/HERMES), NanoSIMS at MNHN Paris and Institut Curie Orsay [1, 3-6, 12, 16, 17]. Recent STXM-XANES analyses were performed at the SOLEIL/HERMES beamline on 4 additional UCAMMs. Results and discussion: The additional STXM-XANES measurements of 4 UCAMM fragments in FIB-sections confirmed the presence of 3 organic phases in UCAMMs : i) an extended (up to tens of µm) smooth N-rich organic phase with a low O content, which is devoid of crystalline phases but can occasionnaly contain Glass Embedded with Metal and Sulfides (GEMS) inclusions; ii) an organic phase similar to the insoluble organic matter (IOM) extracted from ...