Summertime low‐ozone episodes at northern high latitudes

Abstract A pool of low‐ozone air resides in the Arctic stratosphere in summer. Its formation and maintenance arise from a combination of chemical ozone‐destruction and transport processes. The summertime ozone destruction is induced by gas‐phase chemistry dominated by nitrogen and hydrogen catalytic...

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Bibliographic Details
Published in:Quarterly Journal of the Royal Meteorological Society
Main Authors: Orsolini, Y. J., Eskes, H., Hansen, G., Hoppe, U.‐P., Kylling, A., Kyrö, E., Notholt, J., Der A, R. Van, Gathen, P. Von Der
Format: Article in Journal/Newspaper
Language:English
Published: Wiley 2003
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Online Access:http://dx.doi.org/10.1256/qj.02.211
https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1256%2Fqj.02.211
https://rmets.onlinelibrary.wiley.com/doi/pdf/10.1256/qj.02.211
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Summary:Abstract A pool of low‐ozone air resides in the Arctic stratosphere in summer. Its formation and maintenance arise from a combination of chemical ozone‐destruction and transport processes. The summertime ozone destruction is induced by gas‐phase chemistry dominated by nitrogen and hydrogen catalytic cycles, which are efficient due to long summertime insolation at high latitudes. It is shown that, during events referred to as low‐ozone episodes (LOEs), column ozone can locally decrease to values comparable with the seasonal minimum. A combination is used of (i) assimilation of satellite ozone observations from the Global Ozone Monitoring Experiment, (ii) chemical trajectory modelling, and (iii) the gathering of new lidar and in situ ozone observations in the European Arctic in summer 2000. Hence it is shown that such LOEs involve the displacement of the pool of low‐ozone air in the middle stratosphere, which is more dynamic than previously thought and undergoes pronounced meridional excursions, in particular towards northern Europe. The thinner the ozone layer, the more ultraviolet (UV) radiation reaches the ground, where it can impact on human health and ecosystems. Erythemal UV dose enhancements of the order of 10–15% were observed in northern Norway during the LOEs in summer 2000. Copyright © 2003 Royal Meteorological Society