Inelastic Neutron Scattering from Ice and Other Proton-containing Substances
Abstract A brief introduction to neutron scattering is given with special emphasis on the difference between coherent and incoherent contributions. The following report of recent work on ice contains the determination and verification of some phonon dispersion curves, and outlines the state of the a...
Published in: | Journal of Glaciology |
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Main Author: | |
Format: | Article in Journal/Newspaper |
Language: | English |
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Cambridge University Press (CUP)
1978
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Online Access: | http://dx.doi.org/10.1017/s0022143000033438 https://www.cambridge.org/core/services/aop-cambridge-core/content/view/S0022143000033438 |
Summary: | Abstract A brief introduction to neutron scattering is given with special emphasis on the difference between coherent and incoherent contributions. The following report of recent work on ice contains the determination and verification of some phonon dispersion curves, and outlines the state of the art on diffuse scattering due to the proton disorder. Results on “two-dimensional ice” in copper formate tetrahydrate are of great interest as this system exhibits a phase transformation below which the protons are ordered. The study of rotational diffusion and of the tunnel splitting of the rotational ground state of molecules which contain protons is discussed in some detail. These investigations are now possible with very high energy resolution ΔE ≈ 5 × 10 -8 eV (4 • 10-4 cm- 1 or 12 MHz). |
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