Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today

© The Author(s), 2014. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Scientific Reports 4 (2014): 5848, doi:10.1038/srep05848. Interior Antarctica is among the most remote places on Earth and was thought to be beyond...

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Published in:Scientific Reports
Main Authors: McConnell, Joseph R., Maselli, Olivia J., Sigl, Michael, Vallelonga, P., Neumann, T., Anschutz, H., Bales, R. C., Curran, M. A. J., Das, Sarah B., Edwards, R., Kipfstuhl, Sepp, Layman, Lawrence, Thomas, E. R.
Format: Article in Journal/Newspaper
Language:English
Published: Nature Publishing Group 2014
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Online Access:https://hdl.handle.net/1912/6828
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spelling ftwhoas:oai:darchive.mblwhoilibrary.org:1912/6828 2023-05-15T13:53:15+02:00 Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today McConnell, Joseph R. Maselli, Olivia J. Sigl, Michael Vallelonga, P. Neumann, T. Anschutz, H. Bales, R. C. Curran, M. A. J. Das, Sarah B. Edwards, R. Kipfstuhl, Sepp Layman, Lawrence Thomas, E. R. 2014-07-28 application/vnd.ms-excel application/pdf https://hdl.handle.net/1912/6828 en_US eng Nature Publishing Group https://doi.org/10.1038/srep05848 Scientific Reports 4 (2014): 5848 https://hdl.handle.net/1912/6828 doi:10.1038/srep05848 Attribution-NonCommercial-NoDerivatives 4.0 International http://creativecommons.org/licenses/by-nc-nd/4.0/ CC-BY-NC-ND Scientific Reports 4 (2014): 5848 doi:10.1038/srep05848 Article 2014 ftwhoas https://doi.org/10.1038/srep05848 2022-05-28T22:59:09Z © The Author(s), 2014. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Scientific Reports 4 (2014): 5848, doi:10.1038/srep05848. Interior Antarctica is among the most remote places on Earth and was thought to be beyond the reach of human impacts when Amundsen and Scott raced to the South Pole in 1911. Here we show detailed measurements from an extensive array of 16 ice cores quantifying substantial toxic heavy metal lead pollution at South Pole and throughout Antarctica by 1889 – beating polar explorers by more than 22 years. Unlike the Arctic where lead pollution peaked in the 1970s, lead pollution in Antarctica was as high in the early 20th century as at any time since industrialization. The similar timing and magnitude of changes in lead deposition across Antarctica, as well as the characteristic isotopic signature of Broken Hill lead found throughout the continent, suggest that this single emission source in southern Australia was responsible for the introduction of lead pollution into Antarctica at the end of the 19th century and remains a significant source today. An estimated 660 t of industrial lead have been deposited over Antarctica during the past 130 years as a result of mid-latitude industrial emissions, with regional-to-global scale circulation likely modulating aerosol concentrations. Despite abatement efforts, significant lead pollution in Antarctica persists into the 21st century. This work primarily was supported by the U.S. National Science Foundation Division of Polar Programs (research grants 9903744, 0538427, 0538416, 0968391, 1142166, 0632031; instrument grants 0216552, 0421412). Article in Journal/Newspaper Antarc* Antarctic Antarctica Arctic ice core South pole South pole Woods Hole Scientific Community: WHOAS (Woods Hole Open Access Server) Antarctic Arctic South Pole Scientific Reports 4 1
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language English
description © The Author(s), 2014. This article is distributed under the terms of the Creative Commons Attribution License. The definitive version was published in Scientific Reports 4 (2014): 5848, doi:10.1038/srep05848. Interior Antarctica is among the most remote places on Earth and was thought to be beyond the reach of human impacts when Amundsen and Scott raced to the South Pole in 1911. Here we show detailed measurements from an extensive array of 16 ice cores quantifying substantial toxic heavy metal lead pollution at South Pole and throughout Antarctica by 1889 – beating polar explorers by more than 22 years. Unlike the Arctic where lead pollution peaked in the 1970s, lead pollution in Antarctica was as high in the early 20th century as at any time since industrialization. The similar timing and magnitude of changes in lead deposition across Antarctica, as well as the characteristic isotopic signature of Broken Hill lead found throughout the continent, suggest that this single emission source in southern Australia was responsible for the introduction of lead pollution into Antarctica at the end of the 19th century and remains a significant source today. An estimated 660 t of industrial lead have been deposited over Antarctica during the past 130 years as a result of mid-latitude industrial emissions, with regional-to-global scale circulation likely modulating aerosol concentrations. Despite abatement efforts, significant lead pollution in Antarctica persists into the 21st century. This work primarily was supported by the U.S. National Science Foundation Division of Polar Programs (research grants 9903744, 0538427, 0538416, 0968391, 1142166, 0632031; instrument grants 0216552, 0421412).
format Article in Journal/Newspaper
author McConnell, Joseph R.
Maselli, Olivia J.
Sigl, Michael
Vallelonga, P.
Neumann, T.
Anschutz, H.
Bales, R. C.
Curran, M. A. J.
Das, Sarah B.
Edwards, R.
Kipfstuhl, Sepp
Layman, Lawrence
Thomas, E. R.
spellingShingle McConnell, Joseph R.
Maselli, Olivia J.
Sigl, Michael
Vallelonga, P.
Neumann, T.
Anschutz, H.
Bales, R. C.
Curran, M. A. J.
Das, Sarah B.
Edwards, R.
Kipfstuhl, Sepp
Layman, Lawrence
Thomas, E. R.
Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today
author_facet McConnell, Joseph R.
Maselli, Olivia J.
Sigl, Michael
Vallelonga, P.
Neumann, T.
Anschutz, H.
Bales, R. C.
Curran, M. A. J.
Das, Sarah B.
Edwards, R.
Kipfstuhl, Sepp
Layman, Lawrence
Thomas, E. R.
author_sort McConnell, Joseph R.
title Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today
title_short Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today
title_full Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today
title_fullStr Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today
title_full_unstemmed Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today
title_sort antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today
publisher Nature Publishing Group
publishDate 2014
url https://hdl.handle.net/1912/6828
geographic Antarctic
Arctic
South Pole
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Arctic
South Pole
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Antarctic
Antarctica
Arctic
ice core
South pole
South pole
genre_facet Antarc*
Antarctic
Antarctica
Arctic
ice core
South pole
South pole
op_source Scientific Reports 4 (2014): 5848
doi:10.1038/srep05848
op_relation https://doi.org/10.1038/srep05848
Scientific Reports 4 (2014): 5848
https://hdl.handle.net/1912/6828
doi:10.1038/srep05848
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