Radium Inputs Into the Arctic Ocean From Rivers:A Basin-Wide Estimate

• Published in: Journal of Geophysical Research: Oceans
• Main Authors: Bullock, Emma J., Kipp, Lauren, Moore, Willard, Brown, Kristina, Mann, Paul J., Vonk, Jorien E., Zimov, Nikita, Charette, Matthew A.
• Format: Article in Journal/Newspaper
• Language: English
• Published: 2022
• Subjects: Arctic Ocean; radium isotopes; river fluxes; /dk/atira/pure/sustainabledevelopmentgoals/life_below_water; name=SDG 14 - Life Below Water; Arctic; Climate change; Ice; permafrost
• Online Access: https://research.vu.nl/en/publications/78c5622f-98d5-45bb-988c-5cafe8d7eb99; https://doi.org/10.1029/2022JC018964; https://hdl.handle.net/1871.1/78c5622f-98d5-45bb-988c-5cafe8d7eb99; http://www.scopus.com/inward/record.url?scp=85139102927&partnerID=8YFLogxK; http://www.scopus.com/inward/citedby.url?scp=85139102927&partnerID=8YFLogxK

Radium isotopes have been used to trace nutrient, carbon, and trace metal fluxes inputs from ocean margins. However, these approaches require a full accounting of radium sources to the coastal ocean including rivers. Here, we aim to quantify river radium inputs into the Arctic Ocean for the first time for 226 Ra and to refine the estimates for 228 Ra. Using new and existing data, we find that the estimated combined (dissolved plus desorbed) annual 226 Ra and 228 Ra fluxes to the Arctic Ocean are [7.0–9.4] × 10 14 dpm y −1 and [15–18] × 10 14 dpm y −1 , respectively. Of these totals, 44% and 60% of the river 226 Ra and 228 Ra, respectively are from suspended sediment desorption, which were estimated from laboratory incubation experiments. Using Ra isotope data from 20 major rivers around the world, we derived global annual 226 Ra and 228 Ra fluxes of [7.4–17] × 10 15 and [15–27] × 10 15 dpm y −1 , respectively. As climate change spurs rapid Arctic warming, hydrological cycles are intensifying and coastal ice cover and permafrost are diminishing. These river radium inputs to the Arctic Ocean will serve as a valuable baseline as we attempt to understand the changes that warming temperatures are having on fluxes of biogeochemically important elements to the Arctic coastal zone.