Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change?
Can a climate-triggered export of old contaminants from the soil alter the lead (Pb) contaminant burden of subarctic lakes? To address this question, we reconstructed the pollution history of three high latitude lakes situated in a region where a recent climatic shift has occurred. Dated sediment re...
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Online Access: | https://research.vu.nl/en/publications/1f8acfbc-942c-416e-9439-93b0437bc4ce https://doi.org/10.1021/es903025z http://hdl.handle.net/1871.1/1f8acfbc-942c-416e-9439-93b0437bc4ce http://www.scopus.com/inward/record.url?scp=77950411959&partnerID=8YFLogxK http://www.scopus.com/inward/citedby.url?scp=77950411959&partnerID=8YFLogxK |
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ftvuamstcris:oai:research.vu.nl:publications/1f8acfbc-942c-416e-9439-93b0437bc4ce 2023-05-15T17:57:53+02:00 Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change? Jonatan, Klaminder Dan, Hammarlund Ulla, Kokfelt Vonk And, Jorien E. Christian, Bigler 2010-04-01 https://research.vu.nl/en/publications/1f8acfbc-942c-416e-9439-93b0437bc4ce https://doi.org/10.1021/es903025z http://hdl.handle.net/1871.1/1f8acfbc-942c-416e-9439-93b0437bc4ce http://www.scopus.com/inward/record.url?scp=77950411959&partnerID=8YFLogxK http://www.scopus.com/inward/citedby.url?scp=77950411959&partnerID=8YFLogxK eng eng info:eu-repo/semantics/restrictedAccess Jonatan , K , Dan , H , Ulla , K , Vonk And , J E & Christian , B 2010 , ' Lead contamination of subarctic lakes and its response to reduced atmospheric fallout : Can the recovery process be counteracted by the ongoing Climate change? ' , Environmental Science and Technology , vol. 44 , no. 7 , pp. 2335-2340 . https://doi.org/10.1021/es903025z article 2010 ftvuamstcris https://doi.org/10.1021/es903025z 2022-01-17T13:27:25Z Can a climate-triggered export of old contaminants from the soil alter the lead (Pb) contaminant burden of subarctic lakes? To address this question, we reconstructed the pollution history of three high latitude lakes situated in a region where a recent climatic shift has occurred. Dated sediment records were used as archives of past Pb inputs to the lakes, where the difference in the 206 Pb/ 207 Pb ratio between atmospheric contaminants ( 206 Pb/ 207 Pb ratio <1.16) and geogenic Pb in the catchment soil ( 206 Pb/ 207 Pb ratio > 1.22) were used to trace fluxes of Pb contaminants. Lead contaminants were found in sediments deposited since Roman times. A significant export of Pb from the soil contaminant pool is indicated in two of the lakes surrounded by near-shore permafrost soils. Here, levels of Pb contaminants and 206 Pb/ 207 Pb ratios of sediments deposited after the 1970s appear not to have been strongly affected by the ≥ 90% reduction in atmospheric deposition rates and increasing 206 Pb/ 207 Pb ratios of atmospheric Pb since the 1990s. We concluded that soil processes stimulated by the ongoing climate change at high latitudes might work counteractive to efforts to reduce contaminant levels in subarctic lakes. Article in Journal/Newspaper permafrost Subarctic Vrije Universiteit Amsterdam (VU): Research Portal Environmental Science & Technology 44 7 2335 2340 |
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Open Polar |
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Vrije Universiteit Amsterdam (VU): Research Portal |
op_collection_id |
ftvuamstcris |
language |
English |
description |
Can a climate-triggered export of old contaminants from the soil alter the lead (Pb) contaminant burden of subarctic lakes? To address this question, we reconstructed the pollution history of three high latitude lakes situated in a region where a recent climatic shift has occurred. Dated sediment records were used as archives of past Pb inputs to the lakes, where the difference in the 206 Pb/ 207 Pb ratio between atmospheric contaminants ( 206 Pb/ 207 Pb ratio <1.16) and geogenic Pb in the catchment soil ( 206 Pb/ 207 Pb ratio > 1.22) were used to trace fluxes of Pb contaminants. Lead contaminants were found in sediments deposited since Roman times. A significant export of Pb from the soil contaminant pool is indicated in two of the lakes surrounded by near-shore permafrost soils. Here, levels of Pb contaminants and 206 Pb/ 207 Pb ratios of sediments deposited after the 1970s appear not to have been strongly affected by the ≥ 90% reduction in atmospheric deposition rates and increasing 206 Pb/ 207 Pb ratios of atmospheric Pb since the 1990s. We concluded that soil processes stimulated by the ongoing climate change at high latitudes might work counteractive to efforts to reduce contaminant levels in subarctic lakes. |
format |
Article in Journal/Newspaper |
author |
Jonatan, Klaminder Dan, Hammarlund Ulla, Kokfelt Vonk And, Jorien E. Christian, Bigler |
spellingShingle |
Jonatan, Klaminder Dan, Hammarlund Ulla, Kokfelt Vonk And, Jorien E. Christian, Bigler Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change? |
author_facet |
Jonatan, Klaminder Dan, Hammarlund Ulla, Kokfelt Vonk And, Jorien E. Christian, Bigler |
author_sort |
Jonatan, Klaminder |
title |
Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change? |
title_short |
Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change? |
title_full |
Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change? |
title_fullStr |
Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change? |
title_full_unstemmed |
Lead contamination of subarctic lakes and its response to reduced atmospheric fallout:Can the recovery process be counteracted by the ongoing Climate change? |
title_sort |
lead contamination of subarctic lakes and its response to reduced atmospheric fallout:can the recovery process be counteracted by the ongoing climate change? |
publishDate |
2010 |
url |
https://research.vu.nl/en/publications/1f8acfbc-942c-416e-9439-93b0437bc4ce https://doi.org/10.1021/es903025z http://hdl.handle.net/1871.1/1f8acfbc-942c-416e-9439-93b0437bc4ce http://www.scopus.com/inward/record.url?scp=77950411959&partnerID=8YFLogxK http://www.scopus.com/inward/citedby.url?scp=77950411959&partnerID=8YFLogxK |
genre |
permafrost Subarctic |
genre_facet |
permafrost Subarctic |
op_source |
Jonatan , K , Dan , H , Ulla , K , Vonk And , J E & Christian , B 2010 , ' Lead contamination of subarctic lakes and its response to reduced atmospheric fallout : Can the recovery process be counteracted by the ongoing Climate change? ' , Environmental Science and Technology , vol. 44 , no. 7 , pp. 2335-2340 . https://doi.org/10.1021/es903025z |
op_rights |
info:eu-repo/semantics/restrictedAccess |
op_doi |
https://doi.org/10.1021/es903025z |
container_title |
Environmental Science & Technology |
container_volume |
44 |
container_issue |
7 |
container_start_page |
2335 |
op_container_end_page |
2340 |
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1766166391170269184 |