Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements
International audience We present airborne measurements of carbon dioxide (CO2), carbon monoxide (CO), ozone (O3), equivalent black carbon (EBC) and ultra fine particles over North-Eastern Siberia in July 2008 performed during the YAK-AEROSIB/POLARCAT experiment. During a "golden day" (11...
Published in: | Atmospheric Chemistry and Physics |
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Main Authors: | , , , , , , , , |
Other Authors: | , , , , , , , , , , , , , , , , |
Format: | Article in Journal/Newspaper |
Language: | English |
Published: |
HAL CCSD
2009
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Subjects: | |
Online Access: | https://hal.science/hal-00416203 https://hal.science/hal-00416203/document https://hal.science/hal-00416203/file/acp-9-9315-2009.pdf https://doi.org/10.5194/acp-9-9315-2009 |
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ftutoulouse3hal:oai:HAL:hal-00416203v1 |
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record_format |
openpolar |
institution |
Open Polar |
collection |
Université Toulouse III - Paul Sabatier: HAL-UPS |
op_collection_id |
ftutoulouse3hal |
language |
English |
topic |
[SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] |
spellingShingle |
[SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] Paris, J.-D. Stohl, A. Nédélec, P. Arshinov, M.Yu. Panchenko, M.V. Shmargunov, V.P. Law, Kathy S. Belan, B.D. Ciais, Philippe Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements |
topic_facet |
[SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] |
description |
International audience We present airborne measurements of carbon dioxide (CO2), carbon monoxide (CO), ozone (O3), equivalent black carbon (EBC) and ultra fine particles over North-Eastern Siberia in July 2008 performed during the YAK-AEROSIB/POLARCAT experiment. During a "golden day" (11 July 2008) a number of biomass burning plumes were encountered with CO concentration enhancements of up to 500 ppb relative to a background of 90 ppb. Number concentrations of aerosols in the size range 3.5–200 nm peaked at 4000 cm−3 and the EBC content reached 1.4 μg m−3. These high concentrations were caused by forest fires in the vicinity of the landing airport in Yakutsk where during the descent measurements in fresh smoke could be made. We estimate a combustion efficiency of 90±3% based on CO and CO2 measurements. The emission factor of CO emitted was 59.6±15.2 g CO per kilogram of dry matter burned, suggesting an increase in the average northern hemispheric CO concentration of 3.0–7.2 ppb per million hectares of Siberian forest burned. For BC, we estimate an emission factor of 0.52±0.07 g BC kg−1, comparable to values reported in the literature. The emission ratio of ultra-fine particles (3.5–200 nm) was 26 cm−3 (ppb CO)−1, consistent with other airborne studies. |
author2 |
Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA) ICOS-RAMCES (ICOS-RAMCES) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Norwegian Institute for Air Research (NILU) Laboratoire d'aérologie (LAERO) Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP) Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) V.E. Zuev Institute of Atmospheric Optics (IAO) Siberian Branch of the Russian Academy of Sciences (SB RAS) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) ICOS-ATC (ICOS-ATC) |
format |
Article in Journal/Newspaper |
author |
Paris, J.-D. Stohl, A. Nédélec, P. Arshinov, M.Yu. Panchenko, M.V. Shmargunov, V.P. Law, Kathy S. Belan, B.D. Ciais, Philippe |
author_facet |
Paris, J.-D. Stohl, A. Nédélec, P. Arshinov, M.Yu. Panchenko, M.V. Shmargunov, V.P. Law, Kathy S. Belan, B.D. Ciais, Philippe |
author_sort |
Paris, J.-D. |
title |
Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements |
title_short |
Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements |
title_full |
Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements |
title_fullStr |
Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements |
title_full_unstemmed |
Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements |
title_sort |
wildfire smoke in the siberian arctic in summer: source characterization and plume evolution from airborne measurements |
publisher |
HAL CCSD |
publishDate |
2009 |
url |
https://hal.science/hal-00416203 https://hal.science/hal-00416203/document https://hal.science/hal-00416203/file/acp-9-9315-2009.pdf https://doi.org/10.5194/acp-9-9315-2009 |
genre |
black carbon Yakutsk Siberia |
genre_facet |
black carbon Yakutsk Siberia |
op_source |
ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://hal.science/hal-00416203 Atmospheric Chemistry and Physics, 2009, 9 (23), pp.9315-9327. ⟨10.5194/acp-9-9315-2009⟩ |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-9-9315-2009 hal-00416203 https://hal.science/hal-00416203 https://hal.science/hal-00416203/document https://hal.science/hal-00416203/file/acp-9-9315-2009.pdf doi:10.5194/acp-9-9315-2009 |
op_rights |
info:eu-repo/semantics/OpenAccess |
op_doi |
https://doi.org/10.5194/acp-9-9315-2009 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
9 |
container_issue |
23 |
container_start_page |
9315 |
op_container_end_page |
9327 |
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1810437092710285312 |
spelling |
ftutoulouse3hal:oai:HAL:hal-00416203v1 2024-09-15T17:59:58+00:00 Wildfire smoke in the Siberian Arctic in summer: source characterization and plume evolution from airborne measurements Paris, J.-D. Stohl, A. Nédélec, P. Arshinov, M.Yu. Panchenko, M.V. Shmargunov, V.P. Law, Kathy S. Belan, B.D. Ciais, Philippe Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA) ICOS-RAMCES (ICOS-RAMCES) Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)) Norwegian Institute for Air Research (NILU) Laboratoire d'aérologie (LAERO) Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP) Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3) Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales Toulouse (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France-Centre National de la Recherche Scientifique (CNRS) V.E. Zuev Institute of Atmospheric Optics (IAO) Siberian Branch of the Russian Academy of Sciences (SB RAS) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) ICOS-ATC (ICOS-ATC) 2009 https://hal.science/hal-00416203 https://hal.science/hal-00416203/document https://hal.science/hal-00416203/file/acp-9-9315-2009.pdf https://doi.org/10.5194/acp-9-9315-2009 en eng HAL CCSD European Geosciences Union info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-9-9315-2009 hal-00416203 https://hal.science/hal-00416203 https://hal.science/hal-00416203/document https://hal.science/hal-00416203/file/acp-9-9315-2009.pdf doi:10.5194/acp-9-9315-2009 info:eu-repo/semantics/OpenAccess ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://hal.science/hal-00416203 Atmospheric Chemistry and Physics, 2009, 9 (23), pp.9315-9327. ⟨10.5194/acp-9-9315-2009⟩ [SDE.ES]Environmental Sciences/Environment and Society [SDE.MCG]Environmental Sciences/Global Changes [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] info:eu-repo/semantics/article Journal articles 2009 ftutoulouse3hal https://doi.org/10.5194/acp-9-9315-2009 2024-06-25T00:23:41Z International audience We present airborne measurements of carbon dioxide (CO2), carbon monoxide (CO), ozone (O3), equivalent black carbon (EBC) and ultra fine particles over North-Eastern Siberia in July 2008 performed during the YAK-AEROSIB/POLARCAT experiment. During a "golden day" (11 July 2008) a number of biomass burning plumes were encountered with CO concentration enhancements of up to 500 ppb relative to a background of 90 ppb. Number concentrations of aerosols in the size range 3.5–200 nm peaked at 4000 cm−3 and the EBC content reached 1.4 μg m−3. These high concentrations were caused by forest fires in the vicinity of the landing airport in Yakutsk where during the descent measurements in fresh smoke could be made. We estimate a combustion efficiency of 90±3% based on CO and CO2 measurements. The emission factor of CO emitted was 59.6±15.2 g CO per kilogram of dry matter burned, suggesting an increase in the average northern hemispheric CO concentration of 3.0–7.2 ppb per million hectares of Siberian forest burned. For BC, we estimate an emission factor of 0.52±0.07 g BC kg−1, comparable to values reported in the literature. The emission ratio of ultra-fine particles (3.5–200 nm) was 26 cm−3 (ppb CO)−1, consistent with other airborne studies. Article in Journal/Newspaper black carbon Yakutsk Siberia Université Toulouse III - Paul Sabatier: HAL-UPS Atmospheric Chemistry and Physics 9 23 9315 9327 |