Aerosol formation in the Antarctic sea-ice region
Particles in the atmosphere, or aerosols, are vital components of many chemical and physical processes including the Earth's radiative balance. The mechanisms of aerosol formation, along with their interactions with clouds and subsequent effect on the radiative balance, are among the largest un...
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ftunivwollongong:oai:ro.uow.edu.au:theses-5545 2023-05-15T13:43:25+02:00 Aerosol formation in the Antarctic sea-ice region Humphries, Ruhi 2015-01-01T08:00:00Z application/pdf https://ro.uow.edu.au/theses/4536 https://ro.uow.edu.au/cgi/viewcontent.cgi?article=5545&context=theses unknown School of Chemistry https://ro.uow.edu.au/theses/4536 https://ro.uow.edu.au/cgi/viewcontent.cgi?article=5545&context=theses University of Wollongong Thesis Collection 1954-2016 Southern Ocean aerosols atmospheric particles atmospheric chemistry atmospheric science Antarctica Southern Hemisphere circulation mercury chemistry thesis 2015 ftunivwollongong 2021-11-08T23:30:26Z Particles in the atmosphere, or aerosols, are vital components of many chemical and physical processes including the Earth's radiative balance. The mechanisms of aerosol formation, along with their interactions with clouds and subsequent effect on the radiative balance, are among the largest uncertainties present in our understanding of the climate system. Recent modelling studies have shown that the greatest gains in reducing these uncertainties will be achieved through the study of pristine, natural aerosol processes. There are very few observations in the Antarctic and Southern Ocean regions. Those that have been made have been primarily limited to boundary layer airmasses at spatially sparse coastal and continental research stations, or to ship-based measurements in the Southern Ocean. The dynamic Antarctic sea ice region, when at its maximum spatial extent, covers more area than the continent itself, however aerosol measurements within this region have only been performed once before. This thesis describes results from atmospheric measurements made on-board Australia’s flagship ice-breaker, Aurora Australis, during a marine science voyage to the sea ice region off the East Antarctic coast during the spring of 2012. Measurements of aerosols and various trace gases were made continually throughout the voyage, resulting in significant advances in the scientific understanding of the region which this research has shown to be atmospherically distinct from adjacent areas. The collected aerosol dataset has two main features. Firstly, background aerosol concentrations were higher than any other previously recorded in the Antarctic and Southern Ocean region. Secondly, a single new particle formation event was observed during the 32 day aerosol record which could not be explained by known nucleation chemistry. Thesis Antarc* Antarctic Antarctica aurora australis Sea ice Southern Ocean University of Wollongong, Australia: Research Online Antarctic Breaker ENVELOPE(-67.257,-67.257,-67.874,-67.874) Southern Ocean The Antarctic |
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Open Polar |
collection |
University of Wollongong, Australia: Research Online |
op_collection_id |
ftunivwollongong |
language |
unknown |
topic |
Southern Ocean aerosols atmospheric particles atmospheric chemistry atmospheric science Antarctica Southern Hemisphere circulation mercury chemistry |
spellingShingle |
Southern Ocean aerosols atmospheric particles atmospheric chemistry atmospheric science Antarctica Southern Hemisphere circulation mercury chemistry Humphries, Ruhi Aerosol formation in the Antarctic sea-ice region |
topic_facet |
Southern Ocean aerosols atmospheric particles atmospheric chemistry atmospheric science Antarctica Southern Hemisphere circulation mercury chemistry |
description |
Particles in the atmosphere, or aerosols, are vital components of many chemical and physical processes including the Earth's radiative balance. The mechanisms of aerosol formation, along with their interactions with clouds and subsequent effect on the radiative balance, are among the largest uncertainties present in our understanding of the climate system. Recent modelling studies have shown that the greatest gains in reducing these uncertainties will be achieved through the study of pristine, natural aerosol processes. There are very few observations in the Antarctic and Southern Ocean regions. Those that have been made have been primarily limited to boundary layer airmasses at spatially sparse coastal and continental research stations, or to ship-based measurements in the Southern Ocean. The dynamic Antarctic sea ice region, when at its maximum spatial extent, covers more area than the continent itself, however aerosol measurements within this region have only been performed once before. This thesis describes results from atmospheric measurements made on-board Australia’s flagship ice-breaker, Aurora Australis, during a marine science voyage to the sea ice region off the East Antarctic coast during the spring of 2012. Measurements of aerosols and various trace gases were made continually throughout the voyage, resulting in significant advances in the scientific understanding of the region which this research has shown to be atmospherically distinct from adjacent areas. The collected aerosol dataset has two main features. Firstly, background aerosol concentrations were higher than any other previously recorded in the Antarctic and Southern Ocean region. Secondly, a single new particle formation event was observed during the 32 day aerosol record which could not be explained by known nucleation chemistry. |
format |
Thesis |
author |
Humphries, Ruhi |
author_facet |
Humphries, Ruhi |
author_sort |
Humphries, Ruhi |
title |
Aerosol formation in the Antarctic sea-ice region |
title_short |
Aerosol formation in the Antarctic sea-ice region |
title_full |
Aerosol formation in the Antarctic sea-ice region |
title_fullStr |
Aerosol formation in the Antarctic sea-ice region |
title_full_unstemmed |
Aerosol formation in the Antarctic sea-ice region |
title_sort |
aerosol formation in the antarctic sea-ice region |
publisher |
School of Chemistry |
publishDate |
2015 |
url |
https://ro.uow.edu.au/theses/4536 https://ro.uow.edu.au/cgi/viewcontent.cgi?article=5545&context=theses |
long_lat |
ENVELOPE(-67.257,-67.257,-67.874,-67.874) |
geographic |
Antarctic Breaker Southern Ocean The Antarctic |
geographic_facet |
Antarctic Breaker Southern Ocean The Antarctic |
genre |
Antarc* Antarctic Antarctica aurora australis Sea ice Southern Ocean |
genre_facet |
Antarc* Antarctic Antarctica aurora australis Sea ice Southern Ocean |
op_source |
University of Wollongong Thesis Collection 1954-2016 |
op_relation |
https://ro.uow.edu.au/theses/4536 https://ro.uow.edu.au/cgi/viewcontent.cgi?article=5545&context=theses |
_version_ |
1766188837620416512 |