Observations of ice nucleating particles over Southern Ocean waters

A likely important feature of the poorly understood aerosol‐cloud interactions over the Southern Ocean (SO) is the dominant role of sea spray aerosol, versus terrestrial aerosol. Ice nucleating particles (INPs), or particles required for heterogeneous ice nucleation, present over the SO have not bee...

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Bibliographic Details
Published in:Geophysical Research Letters
Main Authors: McCluskey, CS, Hill, TCJ, Humphries, RS, Rauker, AM, Moreau, S, Strutton, PG, Chambers, SD, Williams, AG, McRobert, I, Ward, J, Keywood, MD, Harnwell, J, Ponsonby, W, Loh, ZM, Krummel, PB, Protat, A, Kreidenweis, SM, DeMott, PJ
Format: Article in Journal/Newspaper
Language:English
Published: Amer Geophysical Union 2018
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Online Access:https://doi.org/10.1029/2018GL079981
http://ecite.utas.edu.au/128865
Description
Summary:A likely important feature of the poorly understood aerosol‐cloud interactions over the Southern Ocean (SO) is the dominant role of sea spray aerosol, versus terrestrial aerosol. Ice nucleating particles (INPs), or particles required for heterogeneous ice nucleation, present over the SO have not been studied in several decades. In this study, boundary layer aerosol properties and immersion freezing INP number concentrations ( n INPs ) were measured during a ship campaign that occurred south of Australia (down to 53 S) in March‐April 2016. Ocean surface chlorophyll‐ a concentrations ranged from 0.11‐1.77 mg m ‐3 and n INPs were a factor of 100 lower than historical surveys, ranging from 0.38 to 4.6 m ‐3 at ‐20 C. The INP population included organic heat‐stable material, with contributions from heat‐labile material. Lower INP source potentials of SO seawater samples compared to Arctic seawater were consistent with lower ice nucleating site densities in this study compared to north Atlantic air masses.