Year-round record of size-segregated aerosol composition in central Antarctica (Concordia station): Implications for the degree of fractionation of sea-salt particles

International audience The origin of sea-salt aerosol that reaches the high Antarctic plateau and is trapped in snow and ice cores remains still unclear. In particular, the respective role of emissions from the open ocean versus those from the sea-ice surface is not yet quantified. To progress on th...

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Bibliographic Details
Published in:Journal of Geophysical Research
Main Authors: Jourdain, Bruno, Preunkert, Susanne, Cerri, Omar, Castebrunet, Hélène, Udisti, Roberto, Legrand, Michel
Other Authors: Laboratoire de glaciologie et géophysique de l'environnement (LGGE), Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB Université de Savoie Université de Chambéry )-Centre National de la Recherche Scientifique (CNRS)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB Université de Savoie Université de Chambéry )-Centre National de la Recherche Scientifique (CNRS)-Centre National de la Recherche Scientifique (CNRS), Department of Chemistry, Università degli Studi di Firenze = University of Florence (UniFI)
Format: Article in Journal/Newspaper
Language:English
Published: HAL CCSD 2008
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Online Access:https://insu.hal.science/insu-00378451
https://insu.hal.science/insu-00378451/document
https://insu.hal.science/insu-00378451/file/2007JD009584.pdf
https://doi.org/10.1029/2007JD009584
Description
Summary:International audience The origin of sea-salt aerosol that reaches the high Antarctic plateau and is trapped in snow and ice cores remains still unclear. In particular, the respective role of emissions from the open ocean versus those from the sea-ice surface is not yet quantified. To progress on this question, the composition of bulk and size-segregated aerosol was studied in 2006 at the Concordia station (75°S, 123°E) located on the high Antarctic plateau. A depletion of sulfate relative to sodium with respect to the seawater composition is observed on sea-salt aerosol reaching Concordia from April to September. That suggests that in winter, when the sea-salt atmospheric load reaches a maximum, emissions from the sea-ice surface significantly contribute to the sea-salt budget of inland Antarctica.