Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen
International audience Ice core measurements (H 2 O 2 and CH 4 /HCHO) and modeling studies indicate a change in the oxidation capacity of the atmosphere since the onset of the Industrial Revolution due to increases in fossil fuel burning emissions [e.g., Lelieveld et al. , 2002 Hauglustaine and Bras...
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Online Access: | https://hal.science/hal-04418348 https://hal.science/hal-04418348/document https://hal.science/hal-04418348/file/Journal%20of%20Geophysical%20Research%20Atmospheres%20-%202004%20-%20Alexander%20-%20Impact%20of%20preindustrial%20biomass%E2%80%90burning%20emissions%20on%20the.pdf https://doi.org/10.1029/2003JD004218 |
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ftunivsavoie:oai:HAL:hal-04418348v1 2024-04-28T08:21:18+00:00 Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen Alexander, B. Savarino, J. Kreutz, K. Thiemens, M. Department of Chemistry, UCSD University of California San Diego (UC San Diego) University of California (UC)-University of California (UC) Laboratoire de glaciologie et géophysique de l'environnement (LGGE) Observatoire des Sciences de l'Univers de Grenoble (OSUG) Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB Université de Savoie Université de Chambéry )-Centre National de la Recherche Scientifique (CNRS)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB Université de Savoie Université de Chambéry )-Centre National de la Recherche Scientifique (CNRS)-Centre National de la Recherche Scientifique (CNRS) 2004-04-17 https://hal.science/hal-04418348 https://hal.science/hal-04418348/document https://hal.science/hal-04418348/file/Journal%20of%20Geophysical%20Research%20Atmospheres%20-%202004%20-%20Alexander%20-%20Impact%20of%20preindustrial%20biomass%E2%80%90burning%20emissions%20on%20the.pdf https://doi.org/10.1029/2003JD004218 en eng HAL CCSD American Geophysical Union info:eu-repo/semantics/altIdentifier/doi/10.1029/2003JD004218 hal-04418348 https://hal.science/hal-04418348 https://hal.science/hal-04418348/document https://hal.science/hal-04418348/file/Journal%20of%20Geophysical%20Research%20Atmospheres%20-%202004%20-%20Alexander%20-%20Impact%20of%20preindustrial%20biomass%E2%80%90burning%20emissions%20on%20the.pdf doi:10.1029/2003JD004218 info:eu-repo/semantics/OpenAccess ISSN: 2169-897X EISSN: 2169-8996 Journal of Geophysical Research: Atmospheres https://hal.science/hal-04418348 Journal of Geophysical Research: Atmospheres, 2004, 109 (D8), ⟨10.1029/2003JD004218⟩ [SDE]Environmental Sciences info:eu-repo/semantics/article Journal articles 2004 ftunivsavoie https://doi.org/10.1029/2003JD004218 2024-04-11T00:24:45Z International audience Ice core measurements (H 2 O 2 and CH 4 /HCHO) and modeling studies indicate a change in the oxidation capacity of the atmosphere since the onset of the Industrial Revolution due to increases in fossil fuel burning emissions [e.g., Lelieveld et al. , 2002 Hauglustaine and Brasseur , 2001 Wang and Jacob , 1998 Staffelbach et al. , 1991 ]. The mass‐independent fractionation (MIF) in the oxygen isotopes of sulfate and nitrate from a Greenland ice core reveal that biomass‐burning events in North America just prior to the Industrial Revolution significantly impacted the oxidation pathways of sulfur and nitrogen species deposited in Greenland ice. This finding highlights the importance of biomass‐burning emissions for atmospheric chemistry in preindustrial North America and warrants the inclusion of this impact in modeling studies estimating changes in atmospheric oxidant chemistry since the Industrial Revolution, particularly when using paleo‐oxidant data as a reference for model evaluation. Article in Journal/Newspaper Greenland Greenland ice core ice core Université Savoie Mont Blanc: HAL Journal of Geophysical Research: Atmospheres 109 D8 |
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Open Polar |
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Université Savoie Mont Blanc: HAL |
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ftunivsavoie |
language |
English |
topic |
[SDE]Environmental Sciences |
spellingShingle |
[SDE]Environmental Sciences Alexander, B. Savarino, J. Kreutz, K. Thiemens, M. Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen |
topic_facet |
[SDE]Environmental Sciences |
description |
International audience Ice core measurements (H 2 O 2 and CH 4 /HCHO) and modeling studies indicate a change in the oxidation capacity of the atmosphere since the onset of the Industrial Revolution due to increases in fossil fuel burning emissions [e.g., Lelieveld et al. , 2002 Hauglustaine and Brasseur , 2001 Wang and Jacob , 1998 Staffelbach et al. , 1991 ]. The mass‐independent fractionation (MIF) in the oxygen isotopes of sulfate and nitrate from a Greenland ice core reveal that biomass‐burning events in North America just prior to the Industrial Revolution significantly impacted the oxidation pathways of sulfur and nitrogen species deposited in Greenland ice. This finding highlights the importance of biomass‐burning emissions for atmospheric chemistry in preindustrial North America and warrants the inclusion of this impact in modeling studies estimating changes in atmospheric oxidant chemistry since the Industrial Revolution, particularly when using paleo‐oxidant data as a reference for model evaluation. |
author2 |
Department of Chemistry, UCSD University of California San Diego (UC San Diego) University of California (UC)-University of California (UC) Laboratoire de glaciologie et géophysique de l'environnement (LGGE) Observatoire des Sciences de l'Univers de Grenoble (OSUG) Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB Université de Savoie Université de Chambéry )-Centre National de la Recherche Scientifique (CNRS)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Savoie Mont Blanc (USMB Université de Savoie Université de Chambéry )-Centre National de la Recherche Scientifique (CNRS)-Centre National de la Recherche Scientifique (CNRS) |
format |
Article in Journal/Newspaper |
author |
Alexander, B. Savarino, J. Kreutz, K. Thiemens, M. |
author_facet |
Alexander, B. Savarino, J. Kreutz, K. Thiemens, M. |
author_sort |
Alexander, B. |
title |
Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen |
title_short |
Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen |
title_full |
Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen |
title_fullStr |
Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen |
title_full_unstemmed |
Impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen |
title_sort |
impact of preindustrial biomass‐burning emissions on the oxidation pathways of tropospheric sulfur and nitrogen |
publisher |
HAL CCSD |
publishDate |
2004 |
url |
https://hal.science/hal-04418348 https://hal.science/hal-04418348/document https://hal.science/hal-04418348/file/Journal%20of%20Geophysical%20Research%20Atmospheres%20-%202004%20-%20Alexander%20-%20Impact%20of%20preindustrial%20biomass%E2%80%90burning%20emissions%20on%20the.pdf https://doi.org/10.1029/2003JD004218 |
genre |
Greenland Greenland ice core ice core |
genre_facet |
Greenland Greenland ice core ice core |
op_source |
ISSN: 2169-897X EISSN: 2169-8996 Journal of Geophysical Research: Atmospheres https://hal.science/hal-04418348 Journal of Geophysical Research: Atmospheres, 2004, 109 (D8), ⟨10.1029/2003JD004218⟩ |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.1029/2003JD004218 hal-04418348 https://hal.science/hal-04418348 https://hal.science/hal-04418348/document https://hal.science/hal-04418348/file/Journal%20of%20Geophysical%20Research%20Atmospheres%20-%202004%20-%20Alexander%20-%20Impact%20of%20preindustrial%20biomass%E2%80%90burning%20emissions%20on%20the.pdf doi:10.1029/2003JD004218 |
op_rights |
info:eu-repo/semantics/OpenAccess |
op_doi |
https://doi.org/10.1029/2003JD004218 |
container_title |
Journal of Geophysical Research: Atmospheres |
container_volume |
109 |
container_issue |
D8 |
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1797583717587222528 |