The unprecedented 2017-2018 stratospheric smoke event: decay phase and aerosol properties observed with the EARLINET

• Published in: Atmospheric Chemistry and Physics
• Main Authors: Baars, Holger, Ansmann, Albert, Ohneiser, Kevin, Haarig, Moritz, Engelmann, Ronny, Althausen, Dietrich, Hanssen, Ingrid, Gausa, Michael, Pietruczuk, Aleksander, Szkop, Artur, Stachlewska, Iwona S., Wang, Dongxiang, Reichardt, Jens, Skupin, Annett, Mattis, Ina, Trickl, Thomas, Vogelmann, Hannes, Navas-Guzmán, Francisco, Haefele, Alexander, Acheson, Karen, Ruth, Albert A., Tatarov, Boyan, Müller, Detlef, Hu, Qiaoyun, Podvin, Thierry, Goloub, Philippe, Veselovskii, Igor, Pietras, Christophe, Haeffelin, Martial, Fréville, Patrick, Sicard, Michaël, Comerón, Adolfo, Fernández García, Alfonso Javier, Molero Menéndez, Francisco, Córdoba-Jabonero, Carmen, Guerrero-Rascado, Juan Luis, Alados-Arboledas, Lucas, Bortoli, Daniele, João Costa, Maria, Dionisi, Davide, Liberti, Gian Luigi, Wang, Xuan, Sannino, Alessia, Papagiannopoulos, Nikolaos, Boselli, Antonella, Mona, Lucia, d'Amico, Giuseppe, Romano, Salvatore, Perrone, Maria Rita, Belegante, Livio
• Other Authors: Laboratoire d’Optique Atmosphérique - UMR 8518 (LOA), Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Météorologie Dynamique (UMR 8539) (LMD), Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-École des Ponts ParisTech (ENPC)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Observatoire de Physique du Globe de Clermont-Ferrand (OPGC), Institut national des sciences de l'Univers (INSU - CNRS)-Université Clermont Auvergne 2017-2020 (UCA 2017-2020 )-Centre National de la Recherche Scientifique (CNRS)
• Format: Article in Journal/Newspaper
• Language: English
• Published: HAL CCSD 2019
• Subjects: [SDU]Sciences of the Universe [physics]; Canada; Norway; Northern Norway
• Online Access: https://hal-insu.archives-ouvertes.fr/insu-03686269; https://hal-insu.archives-ouvertes.fr/insu-03686269/document; https://hal-insu.archives-ouvertes.fr/insu-03686269/file/acp-19-15183-2019.pdf; https://doi.org/10.5194/acp-19-15183-2019

International audience Six months of stratospheric aerosol observations with the European Aerosol Research Lidar Network (EARLINET) from August 2017 to January 2018 are presented. The decay phase of an unprecedented, record-breaking stratospheric perturbation caused by wildfire smoke is reported and discussed in terms of geometrical, optical, and microphysical aerosol properties. Enormous amounts of smoke were injected into the upper troposphere and lower stratosphere over fire areas in western Canada on 12 August 2017 during strong thunderstorm-pyrocumulonimbus activity. The stratospheric fire plumes spread over the entire Northern Hemisphere in the following weeks and months. Twenty-eight European lidar stations from northern Norway to southern Portugal and the eastern Mediterranean monitored the strong stratospheric perturbation on a continental scale. The main smoke layer (over central, western, southern, and eastern Europe) was found at heights between 15 and 20 km since September 2017 (about 2 weeks after entering the stratosphere). Thin layers of smoke were detected at heights of up to 22-23 km. The stratospheric aerosol optical thickness at 532 nm decreased from values > 0.25 on 21-23 August 2017 to 0.005-0.03 until 5-10 September and was mainly 0.003-0.004 from October to December 2017 and thus was still significantly above the stratospheric background (0.001-0.002). Stratospheric particle extinction coefficients (532 nm) were as high as 50-200 Mm -1 until the beginning of September and on the order of 1 Mm -1 (0.5-5 Mm -1 ) from October 2017 until the end of January 2018. The corresponding layer mean particle mass concentration was on the order of 0.05-0.5 µg m -3 over these months. Soot particles (light-absorbing carbonaceous particles) are efficient ice-nucleating particles (INPs) at upper tropospheric (cirrus) temperatures and available to influence cirrus formation when entering the tropopause from above. We estimated INP concentrations of 50-500 L -1 until the first days in September and ...