Oceanic Radiocarbon Between Antarctica and South Africa Along Woce Section 16 at 30°E

• Published in: Radiocarbon
• Main Authors: Leboucher, Viviane, Orr, James C., Jean-Baptiste, Philippe, Arnold, Maurice, Monfray, Patrick, Tisnérat-Laborde, Nadine, Poisson, Alain, Duplessy, Jean-Claude
• Other Authors: Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Centre européen de recherche et d'enseignement des géosciences de l'environnement (CEREGE), Institut de Recherche pour le Développement (IRD)-Institut National de la Recherche Agronomique (INRA)-Aix Marseille Université (AMU)-Collège de France (CdF (institution))-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Géochrononologie Traceurs Archéométrie (GEOTRAC), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Physique et Chimie Marines (LPCM), Université Pierre et Marie Curie - Paris 6 (UPMC)-Centre National de la Recherche Scientifique (CNRS), Paléocéanographie (PALEOCEAN)
• Format: Article in Journal/Newspaper
• Language: English
• Published: HAL CCSD 1999
• Subjects: [SDU.OCEAN]Sciences of the Universe [physics]/Ocean; Atmosphere; [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces; environment; Antarctic; Pacific; Southern Ocean; The Antarctic; Antarc*; Antarctica
• Online Access: https://hal.science/hal-02500995; https://hal.science/hal-02500995/document; https://hal.science/hal-02500995/file/oceanic-radiocarbon-between-antarctica-and-south-africa-along-woce-section-16-at-30-e-div.pdf; https://doi.org/10.1017/S0033822200019330

International audience Accelerator mass spectrometry (AMS) radiocarbon measurements were made on 120 samples collected between Antarctica and South Africa along 30°E during the WOCE-France CIVA 1 campaign in February 1993. Our principal objective was to complement the Southern Ocean's sparse existing data set in order to improve the 14C benchmark used for validating ocean carbon-cycle models, which disagree considerably in this region. Measured 14C is consistent with the 0-S characteristics of CIVA1. Antarctic Intermediate Water (AAIW) forming north of the Polar Front (PF) is rich in'4C, whereas surface waters south of the PF are depleted in 14C. A distinct old 14C signal was found for the contribution of the Pacific Deep Water (PDW) to the return flow of Circumpolar Deep Waters (CDW). Comparison to previous measurements shows a 4C decrease in surface waters, consistent with northward displacement of surface waters, replacement by old deep waters upwelled at the Antarctic Divergence, and atmospheric decline in 14C. Conversely, an increase was found in deeper layers, in the AAIW. Large uncertainties, associated with previous methods for separating natural and bomb 14C when in the Southern Ocean south of 45°S, motivated us to develop a new approach that relies on a simple mixing model and on chlorofluorocarbon (CFC) measurements also taken during CIVA1. This approach leads to inventories for CIVA1 that are equal to or higher than those calculated with previous methods. Differences between old and new methods are especially high south of approximately 55°S, where bomb 14C inventories are relatively modest.