Volcanic aerosol optical properties and phase partitioning behavior after long-range advection characterized by UV-Lidar measurements

• Published in: Atmospheric Environment
• Main Authors: Miffre, Alain, David, Gregory, Thomas, Benjamin, Rairoux, Patrick, Fjaeraa, A. M., Kristiansen, N. I., Stohl, A.
• Other Authors: Spectrométrie et Télédétection de l'Atmosphère, Laboratoire de Spectrométrie Ionique et Moléculaire (LASIM), Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS)-Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS), Norwegian Institute for Air Research (NILU)
• Format: Article in Journal/Newspaper
• Language: English
• Published: HAL CCSD 2011
• Subjects: Volcanic ash; Lidar; Depolarization; Dispersion model; Eyjafjallajökull; Iceland
• Online Access: https://hal.science/hal-00676487; https://doi.org/10.1016/j.atmosenv.2011.03.057

International audience In this paper, an UV-polarization Lidar is used to study the optical properties of volcanic aerosol in the troposphere. The particles were released by the mid-April 2010 eruption of the Eyjafjallajökull volcano (63.63°N, 19.62°W, Iceland) and passed in the troposphere above Lyon (45.76°N, 4.83°E, France) after advection over 2600 km. The FLEXPART particle dispersion model was applied to simulate the volcanic ash transport from Iceland to South West Europe, at the border of the air traffic closure area. Time-altitude plots of FLEXPART ash concentrations as well as of aerosol backscattering are presented, showing the arrival of volcanic particles in the troposphere above Lyon and their mixing into the planetary boundary layer. The particle UV-backscattering coefficient was typically 4 Mm−1 sr−1 and highly sensitive and accurate particle UV-depolarization measurements were performed, with depolarization ranging from a few to 44%. After few days long-range transport, observed ash particles are still non spherical. The observed variations of the backscattering and depolarization coefficients can be attributed to variations in the volcanic particles content. Ash mass concentrations are then retrieved. Moreover, a partitioning into spherical and non spherical particles is evaluated from number concentration ratios between solid ash particles and spherical hydrated sulfate particles. The microphysical properties of volcanic particles can thus be studied by associating an UV-polarization remote sensing instrument with a numerical volcanic ash dispersion model. Highlights - Volcanic ash particles concentration is measured by ground-based Lidar in troposphere. - Coupling with FLEXPART ash transport model allows to identify volcanic ash particles. - Precise UV-depolarization data allows to discern spherical/non spherical particles. - Phase partitioning between non spherical ash and spherical sulfates is thus evaluated. - After long-range advection, PBL ash particles are low concentrated and still ...