Reconstruction of flux and altitude of volcanic SO 2 emissions from satellite observations: implications for volcanological and atmospherical studies.

• Main Authors: Boichu, Marie, Clarisse, Lieven, Péré, Jean-Christophe, Herbin, Hervé, Goloub, Philippe, Thieuleux, François, Khvorostyanov, Dmitry, Ducos, Fabrice, Clerbaux, Cathy, Tanré, Didier
• Other Authors: Laboratoire d’Optique Atmosphérique - UMR 8518 (LOA), Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique, Université libre de Bruxelles (ULB), Interactions Aérosols Rayonnement (IAR), Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Météorologie Dynamique (UMR 8539) (LMD), Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-École des Ponts ParisTech (ENPC)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL), TROPO - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)
• Format: Conference Object
• Language: English
• Published: HAL CCSD 2016
• Subjects: [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph]; [SDU.STU.VO]Sciences of the Universe [physics]/Earth Sciences/Volcanology; [SDE]Environmental Sciences; Jökull; Etna; Iceland
• Online Access: https://insu.hal.science/insu-01308330

International audience Volcanic sulphur dioxide (SO 2 ) degassing is a crucial indicator of the sub-surface volcanic activity, which is widely used today for volcano monitoring and hazard assessment purposes. Volcanic SO 2 is also important regarding atmospherical studies. More easily detectable from space, SO 2 can be used as a proxy of the presence of ash to anticipate air traffic issues caused by explosive eruptions. Moreover, volcanic SO 2 strongly impacts air quality but also climate following its conversion to radiatively-active sulphate aerosols. However, the accurate assessment of these various impacts is currently hampered by the poor knowledge of volcanic SO 2 emissions, which can substantially vary with time, in terms of flux and altitude.To fulfil this need, we propose a strategy relying on satellite observations, which consequently allows for monitoring the eruptive activity of any remote volcano. The method consists in assimilating snapshots of the SO 2 load, provided by infrared or ultraviolet satellite observations, in an inversion scheme that involves the use of a chemistry-transport model to describe the dispersion of SO 2 released in the atmosphere. Applied on Eyjafjalla- jökull (Iceland) and Etna (Italy) eruption case-studies, this procedure allows for retrospectively reconstructing both the flux and altitude of the SO 2 emissions with an hourly resolution. We show the improvement gained in the simulations and forecasts of the location and mass load of volcanic SO 2 clouds using such a detailed reconstruction of emissions.For calibration-validation purpose, we compared our satellite-derived time-series of the SO 2 flux with ground- based observations available on Etna. This comparison indicates a good agreement during ash-poor phases of the eruption. However, large discrepancies are observed during the ash-rich paroxysmal phase as a result of enhanced plume opacity affecting ground-based ultraviolet spectroscopic retrievals. Therefore, the SO 2 emission rate derived from the ground is ...