Light-absorption of dust and elemental carbon in snow in the Indian Himalayas and the Finnish Arctic

• Published in: Atmospheric Measurement Techniques
• Main Authors: Svensson, Jonas, Strom, Johan, Kivekas, Niku, Dkhar, Nathaniel B., Tayal, Shresth, Sharma, Ved P., Jutila, Arttu, Backman, John, Virkkula, Aki, Ruppel, Meri, Hyvarinen, Antti, Kontu, Anna, Hannula, Henna-Reetta, Lepparanta, Matti, Hooda, Rakesh K., Korhola, Atte, Asmi, Eija, Lihavainen, Heikki
• Other Authors: Department of Physics, Ecosystems and Environment Research Programme, Environmental Change Research Unit (ECRU), Institute for Atmospheric and Earth System Research (INAR), Helsinki Institute of Sustainability Science (HELSUS)
• Format: Article in Journal/Newspaper
• Language: English
• Published: COPERNICUS GESELLSCHAFT MBH 2018
• Subjects: BLACK CARBON; ABSORBING IMPURITIES; ICE CORE; THERMAL/OPTICAL ANALYSIS; ATMOSPHERIC AEROSOLS; TIBETAN PLATEAU; SPECTRAL ALBEDO; NORTHERN INDIA; MIXING STATE; PARTICLES; 1172 Environmental sciences; 116 Chemical sciences; Arctic; Indian; albedo; black carbon; ice core
• Online Access: http://hdl.handle.net/10138/233906

Light-absorbing impurities (LAIs) deposited in snow have the potential to substantially affect the snow radiation budget, with subsequent implications for snow melt. To more accurately quantify the snow albedo, the contribution from different LAIs needs to be assessed. Here we estimate the main LAI components, elemental carbon (EC) (as a proxy for black carbon) and mineral dust in snow from the Indian Himalayas and paired the results with snow samples from Arctic Finland. The impurities are collected onto quartz filters and are analyzed thermal-optically for EC, as well as with an additional optical measurement to estimate the light-absorption of dust separately on the filters. Laboratory tests were conducted using substrates containing soot and mineral particles, especially prepared to test the experimental setup. Analyzed ambient snow samples show EC concentrations that are in the same range as presented by previous research, for each respective region. In terms of the mass absorption cross section (MAC) our ambient EC surprisingly had about half of the MAC value compared to our laboratory standard EC (chimney soot), suggesting a less light absorptive EC in the snow, which has consequences for the snow albedo reduction caused by EC. In the Himalayan samples, larger contributions by dust (in the range of 50% or greater for the light absorption caused by the LAI) highlighted the importance of dust acting as a light absorber in the snow. Moreover, EC concentrations in the Indian samples, acquired from a 120 cm deep snow pit (possibly covering the last five years of snow fall), suggest an increase in both EC and dust deposition. This work emphasizes the complexity in determining the snow albedo, showing that LAI concentrations alone might not be sufficient, but additional transient effects on the light-absorbing properties of the EC need to be considered and studied in the snow. Equally as imperative is the confirmation of the spatial and temporal representativeness of these data by comparing data from several and ...