A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques
Immersion freezing is the most relevant heterogeneous ice nucleation mechanism through which ice crystals are formed in mixed-phase clouds. In recent years, an increasing number of laboratory experiments utilizing a variety of instruments have examined immersion freezing activity of atmospherically...
Published in: | Atmospheric Chemistry and Physics |
---|---|
Main Authors: | , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , |
Format: | Article in Journal/Newspaper |
Language: | English |
Published: |
2015
|
Subjects: | |
Online Access: | http://publikationen.ub.uni-frankfurt.de/frontdoor/index/index/docId/37254 https://nbn-resolving.org/urn:nbn:de:hebis:30:3-372542 https://doi.org/10.5194/acp-15-2489-2015 http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015-supplement.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/container.zip |
id |
ftunivfrankfurt:oai:publikationen.ub.uni-frankfurt.de:37254 |
---|---|
record_format |
openpolar |
institution |
Open Polar |
collection |
Publication Server of Goethe University Frankfurt am Main |
op_collection_id |
ftunivfrankfurt |
language |
English |
topic |
ddc:550 |
spellingShingle |
ddc:550 Hiranuma, Naruki Augustin-Bauditz, Stefanie Bingemer, Heinz Budke, Carsten Curtius, Joachim Danielczok, Anja Diehl, Karoline Dreischmeier, Katharina Ebert, Martin Frank, Fabian Hoffmann, Nadine Kandler, Konrad Kiselev, Alexei Koop, Thomas Leisner, Thomas Möhler, Ottmar Nillius, Björn Peckhaus, Andreas Rose, Diana Hader, John D. Hill, Thomas C. Kanji, Zamin A. Kulkarni, Gargi Levin, Ezra J. T. McCluskey, Christina S. Murakami, Masataka Murray, Benjamin J. Niedermeier, Dennis Petters, Markus D. O'Sullivan, Daniel Saito, Atsushi Schill, Gregory P. Tajiri, Takuya Tolbert, Margret A. Welti, André Whale, Thomas F. Wright, Timothy P. Yamashita, Katsuya A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques |
topic_facet |
ddc:550 |
description |
Immersion freezing is the most relevant heterogeneous ice nucleation mechanism through which ice crystals are formed in mixed-phase clouds. In recent years, an increasing number of laboratory experiments utilizing a variety of instruments have examined immersion freezing activity of atmospherically relevant ice-nucleating particles. However, an intercomparison of these laboratory results is a difficult task because investigators have used different ice nucleation (IN) measurement methods to produce these results. A remaining challenge is to explore the sensitivity and accuracy of these techniques and to understand how the IN results are potentially influenced or biased by experimental parameters associated with these techniques. Within the framework of INUIT (Ice Nuclei Research Unit), we distributed an illite-rich sample (illite NX) as a representative surrogate for atmospheric mineral dust particles to investigators to perform immersion freezing experiments using different IN measurement methods and to obtain IN data as a function of particle concentration, temperature (T), cooling rate and nucleation time. A total of 17 measurement methods were involved in the data intercomparison. Experiments with seven instruments started with the test sample pre-suspended in water before cooling, while 10 other instruments employed water vapor condensation onto dry-dispersed particles followed by immersion freezing. The resulting comprehensive immersion freezing data set was evaluated using the ice nucleation active surface-site density, ns, to develop a representative ns(T) spectrum that spans a wide temperature range (−37 °C < T < −11 °C) and covers 9 orders of magnitude in ns. In general, the 17 immersion freezing measurement techniques deviate, within a range of about 8 °C in terms of temperature, by 3 orders of magnitude with respect to ns. In addition, we show evidence that the immersion freezing efficiency expressed in ns of illite NX particles is relatively independent of droplet size, particle mass in ... |
format |
Article in Journal/Newspaper |
author |
Hiranuma, Naruki Augustin-Bauditz, Stefanie Bingemer, Heinz Budke, Carsten Curtius, Joachim Danielczok, Anja Diehl, Karoline Dreischmeier, Katharina Ebert, Martin Frank, Fabian Hoffmann, Nadine Kandler, Konrad Kiselev, Alexei Koop, Thomas Leisner, Thomas Möhler, Ottmar Nillius, Björn Peckhaus, Andreas Rose, Diana Hader, John D. Hill, Thomas C. Kanji, Zamin A. Kulkarni, Gargi Levin, Ezra J. T. McCluskey, Christina S. Murakami, Masataka Murray, Benjamin J. Niedermeier, Dennis Petters, Markus D. O'Sullivan, Daniel Saito, Atsushi Schill, Gregory P. Tajiri, Takuya Tolbert, Margret A. Welti, André Whale, Thomas F. Wright, Timothy P. Yamashita, Katsuya |
author_facet |
Hiranuma, Naruki Augustin-Bauditz, Stefanie Bingemer, Heinz Budke, Carsten Curtius, Joachim Danielczok, Anja Diehl, Karoline Dreischmeier, Katharina Ebert, Martin Frank, Fabian Hoffmann, Nadine Kandler, Konrad Kiselev, Alexei Koop, Thomas Leisner, Thomas Möhler, Ottmar Nillius, Björn Peckhaus, Andreas Rose, Diana Hader, John D. Hill, Thomas C. Kanji, Zamin A. Kulkarni, Gargi Levin, Ezra J. T. McCluskey, Christina S. Murakami, Masataka Murray, Benjamin J. Niedermeier, Dennis Petters, Markus D. O'Sullivan, Daniel Saito, Atsushi Schill, Gregory P. Tajiri, Takuya Tolbert, Margret A. Welti, André Whale, Thomas F. Wright, Timothy P. Yamashita, Katsuya |
author_sort |
Hiranuma, Naruki |
title |
A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques |
title_short |
A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques |
title_full |
A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques |
title_fullStr |
A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques |
title_full_unstemmed |
A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques |
title_sort |
comprehensive laboratory study on the immersion freezing behavior of illite nx particles : a comparison of 17 ice nucleation measurement techniques |
publishDate |
2015 |
url |
http://publikationen.ub.uni-frankfurt.de/frontdoor/index/index/docId/37254 https://nbn-resolving.org/urn:nbn:de:hebis:30:3-372542 https://doi.org/10.5194/acp-15-2489-2015 http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015-supplement.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/container.zip |
genre |
inuit |
genre_facet |
inuit |
op_relation |
http://publikationen.ub.uni-frankfurt.de/frontdoor/index/index/docId/37254 urn:nbn:de:hebis:30:3-372542 https://nbn-resolving.org/urn:nbn:de:hebis:30:3-372542 https://doi.org/10.5194/acp-15-2489-2015 http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015-supplement.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/container.zip |
op_rights |
http://creativecommons.org/licenses/by/3.0/de/deed.de info:eu-repo/semantics/openAccess |
op_doi |
https://doi.org/10.5194/acp-15-2489-2015 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
15 |
container_issue |
5 |
container_start_page |
2489 |
op_container_end_page |
2518 |
_version_ |
1775352195460366336 |
spelling |
ftunivfrankfurt:oai:publikationen.ub.uni-frankfurt.de:37254 2023-08-27T04:10:17+02:00 A comprehensive laboratory study on the immersion freezing behavior of illite NX particles : a comparison of 17 ice nucleation measurement techniques Hiranuma, Naruki Augustin-Bauditz, Stefanie Bingemer, Heinz Budke, Carsten Curtius, Joachim Danielczok, Anja Diehl, Karoline Dreischmeier, Katharina Ebert, Martin Frank, Fabian Hoffmann, Nadine Kandler, Konrad Kiselev, Alexei Koop, Thomas Leisner, Thomas Möhler, Ottmar Nillius, Björn Peckhaus, Andreas Rose, Diana Hader, John D. Hill, Thomas C. Kanji, Zamin A. Kulkarni, Gargi Levin, Ezra J. T. McCluskey, Christina S. Murakami, Masataka Murray, Benjamin J. Niedermeier, Dennis Petters, Markus D. O'Sullivan, Daniel Saito, Atsushi Schill, Gregory P. Tajiri, Takuya Tolbert, Margret A. Welti, André Whale, Thomas F. Wright, Timothy P. Yamashita, Katsuya 2015-03-06 application/pdf application/octet-stream http://publikationen.ub.uni-frankfurt.de/frontdoor/index/index/docId/37254 https://nbn-resolving.org/urn:nbn:de:hebis:30:3-372542 https://doi.org/10.5194/acp-15-2489-2015 http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015-supplement.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/container.zip eng eng http://publikationen.ub.uni-frankfurt.de/frontdoor/index/index/docId/37254 urn:nbn:de:hebis:30:3-372542 https://nbn-resolving.org/urn:nbn:de:hebis:30:3-372542 https://doi.org/10.5194/acp-15-2489-2015 http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/acp-15-2489-2015-supplement.pdf http://publikationen.ub.uni-frankfurt.de/files/37254/container.zip http://creativecommons.org/licenses/by/3.0/de/deed.de info:eu-repo/semantics/openAccess ddc:550 article doc-type:article 2015 ftunivfrankfurt https://doi.org/10.5194/acp-15-2489-2015 2023-08-06T22:40:43Z Immersion freezing is the most relevant heterogeneous ice nucleation mechanism through which ice crystals are formed in mixed-phase clouds. In recent years, an increasing number of laboratory experiments utilizing a variety of instruments have examined immersion freezing activity of atmospherically relevant ice-nucleating particles. However, an intercomparison of these laboratory results is a difficult task because investigators have used different ice nucleation (IN) measurement methods to produce these results. A remaining challenge is to explore the sensitivity and accuracy of these techniques and to understand how the IN results are potentially influenced or biased by experimental parameters associated with these techniques. Within the framework of INUIT (Ice Nuclei Research Unit), we distributed an illite-rich sample (illite NX) as a representative surrogate for atmospheric mineral dust particles to investigators to perform immersion freezing experiments using different IN measurement methods and to obtain IN data as a function of particle concentration, temperature (T), cooling rate and nucleation time. A total of 17 measurement methods were involved in the data intercomparison. Experiments with seven instruments started with the test sample pre-suspended in water before cooling, while 10 other instruments employed water vapor condensation onto dry-dispersed particles followed by immersion freezing. The resulting comprehensive immersion freezing data set was evaluated using the ice nucleation active surface-site density, ns, to develop a representative ns(T) spectrum that spans a wide temperature range (−37 °C < T < −11 °C) and covers 9 orders of magnitude in ns. In general, the 17 immersion freezing measurement techniques deviate, within a range of about 8 °C in terms of temperature, by 3 orders of magnitude with respect to ns. In addition, we show evidence that the immersion freezing efficiency expressed in ns of illite NX particles is relatively independent of droplet size, particle mass in ... Article in Journal/Newspaper inuit Publication Server of Goethe University Frankfurt am Main Atmospheric Chemistry and Physics 15 5 2489 2518 |