Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study
Depending on the magnitude of their eruptions, volcanoes impact the atmosphere at various temporal and spatial scales. The volcanic source remains a major unknown to rigorously assess these impacts. At the scale of an eruption, the limited knowledge of source parameters, including time-variations of...
Published in: | Atmospheric Chemistry and Physics |
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Main Authors: | , , , , , , |
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Format: | Article in Journal/Newspaper |
Language: | English |
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HAL CCSD
2013
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Online Access: | https://hal.science/hal-00799237 https://hal.science/hal-00799237/document https://hal.science/hal-00799237/file/acp-13-8569-2013.pdf https://doi.org/10.5194/acp-13-8569-2013 |
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Université de Versailles Saint-Quentin-en-Yvelines: HAL-UVSQ |
op_collection_id |
ftuniversailles |
language |
English |
topic |
[SDU.STU.VO]Sciences of the Universe [physics]/Earth Sciences/Volcanology [SDE.MCG]Environmental Sciences/Global Changes |
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[SDU.STU.VO]Sciences of the Universe [physics]/Earth Sciences/Volcanology [SDE.MCG]Environmental Sciences/Global Changes Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
topic_facet |
[SDU.STU.VO]Sciences of the Universe [physics]/Earth Sciences/Volcanology [SDE.MCG]Environmental Sciences/Global Changes |
description |
Depending on the magnitude of their eruptions, volcanoes impact the atmosphere at various temporal and spatial scales. The volcanic source remains a major unknown to rigorously assess these impacts. At the scale of an eruption, the limited knowledge of source parameters, including time-variations of erupted mass flux and emission profile, currently represents the greatest issue that limits the reliability of volcanic cloud forecasts. Today, a growing number of satellite and remote sensing observations of distant plumes are becoming available, bringing indirect information on these source terms. Here, we develop an inverse modeling approach combining satellite observations of the volcanic plume with an Eulerian regional chemistry-transport model (CHIMERE) to better characterise the volcanic SO2 emissions during an eruptive crisis. The May 2010 eruption of Eyjafjallajökull is a perfect case-study to apply this method as the volcano emitted substantial amounts of SO2 during more than a month. We take advantage of the SO2 column amounts provided by a vast set of IASI (Infrared Atmospheric Sounding Interferometer) satellite images to reconstruct retrospectively the time-series of the mid-tropospheric SO2 flux emitted by the volcano with a temporal resolution of ~2 h, spanning the period from 1 to 12 May 2010. The initialisation of chemistry-transport modelling with this reconstructed source allows for a reliable simulation of the evolution of the long-lived tropospheric SO2 cloud over thousands of kilometres. Heterogeneities within the plume, which mainly result from the temporal variability of the emissions, are correctly tracked over a time scale of a week. The robustness of our approach is also demonstrated by the broad similarities between the SO2 flux history determined by this study and the ash discharge behaviour estimated by other means during the phases of high explosive activity at Eyjafjallajökull in May 2010. Finally, we show how a sequential IASI data assimilation allows for a substantial improvement in ... |
author2 |
Laboratoire de Météorologie Dynamique (UMR 8539) (LMD) Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-École des Ponts ParisTech (ENPC)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris École normale supérieure - Paris (ENS-PSL) Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-École normale supérieure - Paris (ENS-PSL) Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL) Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique Université libre de Bruxelles (ULB) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) |
format |
Article in Journal/Newspaper |
author |
Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François |
author_facet |
Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François |
author_sort |
Boichu, Marie |
title |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_short |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_full |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_fullStr |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_full_unstemmed |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_sort |
inverting for volcanic so2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 eyjafjallajökull eruption case-study |
publisher |
HAL CCSD |
publishDate |
2013 |
url |
https://hal.science/hal-00799237 https://hal.science/hal-00799237/document https://hal.science/hal-00799237/file/acp-13-8569-2013.pdf https://doi.org/10.5194/acp-13-8569-2013 |
genre |
Eyjafjallajökull |
genre_facet |
Eyjafjallajökull |
op_source |
ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://hal.science/hal-00799237 Atmospheric Chemistry and Physics, 2013, 13 (17), pp.8569-8584. ⟨10.5194/acp-13-8569-2013⟩ |
op_relation |
info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-13-8569-2013 hal-00799237 https://hal.science/hal-00799237 https://hal.science/hal-00799237/document https://hal.science/hal-00799237/file/acp-13-8569-2013.pdf doi:10.5194/acp-13-8569-2013 |
op_rights |
info:eu-repo/semantics/OpenAccess |
op_doi |
https://doi.org/10.5194/acp-13-8569-2013 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
13 |
container_issue |
17 |
container_start_page |
8569 |
op_container_end_page |
8584 |
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1799479539873611776 |
spelling |
ftuniversailles:oai:HAL:hal-00799237v1 2024-05-19T07:39:57+00:00 Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François Laboratoire de Météorologie Dynamique (UMR 8539) (LMD) Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-École des Ponts ParisTech (ENPC)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris École normale supérieure - Paris (ENS-PSL) Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-École normale supérieure - Paris (ENS-PSL) Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL) Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique Université libre de Bruxelles (ULB) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) 2013 https://hal.science/hal-00799237 https://hal.science/hal-00799237/document https://hal.science/hal-00799237/file/acp-13-8569-2013.pdf https://doi.org/10.5194/acp-13-8569-2013 en eng HAL CCSD European Geosciences Union info:eu-repo/semantics/altIdentifier/doi/10.5194/acp-13-8569-2013 hal-00799237 https://hal.science/hal-00799237 https://hal.science/hal-00799237/document https://hal.science/hal-00799237/file/acp-13-8569-2013.pdf doi:10.5194/acp-13-8569-2013 info:eu-repo/semantics/OpenAccess ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics https://hal.science/hal-00799237 Atmospheric Chemistry and Physics, 2013, 13 (17), pp.8569-8584. ⟨10.5194/acp-13-8569-2013⟩ [SDU.STU.VO]Sciences of the Universe [physics]/Earth Sciences/Volcanology [SDE.MCG]Environmental Sciences/Global Changes info:eu-repo/semantics/article Journal articles 2013 ftuniversailles https://doi.org/10.5194/acp-13-8569-2013 2024-04-25T00:37:04Z Depending on the magnitude of their eruptions, volcanoes impact the atmosphere at various temporal and spatial scales. The volcanic source remains a major unknown to rigorously assess these impacts. At the scale of an eruption, the limited knowledge of source parameters, including time-variations of erupted mass flux and emission profile, currently represents the greatest issue that limits the reliability of volcanic cloud forecasts. Today, a growing number of satellite and remote sensing observations of distant plumes are becoming available, bringing indirect information on these source terms. Here, we develop an inverse modeling approach combining satellite observations of the volcanic plume with an Eulerian regional chemistry-transport model (CHIMERE) to better characterise the volcanic SO2 emissions during an eruptive crisis. The May 2010 eruption of Eyjafjallajökull is a perfect case-study to apply this method as the volcano emitted substantial amounts of SO2 during more than a month. We take advantage of the SO2 column amounts provided by a vast set of IASI (Infrared Atmospheric Sounding Interferometer) satellite images to reconstruct retrospectively the time-series of the mid-tropospheric SO2 flux emitted by the volcano with a temporal resolution of ~2 h, spanning the period from 1 to 12 May 2010. The initialisation of chemistry-transport modelling with this reconstructed source allows for a reliable simulation of the evolution of the long-lived tropospheric SO2 cloud over thousands of kilometres. Heterogeneities within the plume, which mainly result from the temporal variability of the emissions, are correctly tracked over a time scale of a week. The robustness of our approach is also demonstrated by the broad similarities between the SO2 flux history determined by this study and the ash discharge behaviour estimated by other means during the phases of high explosive activity at Eyjafjallajökull in May 2010. Finally, we show how a sequential IASI data assimilation allows for a substantial improvement in ... Article in Journal/Newspaper Eyjafjallajökull Université de Versailles Saint-Quentin-en-Yvelines: HAL-UVSQ Atmospheric Chemistry and Physics 13 17 8569 8584 |