Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols
Due to its isolated location, Antarctica is a natural laboratory for studying atmospheric aerosols and pollution in remote areas. Here, we determined levoglucosan and phenolic compounds (PCs) at diverse Antarctic sites: on the plateau, a coastal station and during an oceanographic cruise. Levoglucos...
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Online Access: | http://hdl.handle.net/10278/3680486 https://doi.org/10.1016/j.scitotenv.2015.11.166 |
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ftuniveneziairis:oai:iris.unive.it:10278/3680486 2024-04-14T08:04:02+00:00 Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols ZANGRANDO, Roberta BARBARO, ELENA VECCHIATO, MARCO KEHRWALD, NATALIE MARIE BARBANTE, Carlo GAMBARO, Andrea Zangrando, Roberta Barbaro, Elena Vecchiato, Marco Kehrwald, NATALIE MARIE Barbante, Carlo Gambaro, Andrea 2016 http://hdl.handle.net/10278/3680486 https://doi.org/10.1016/j.scitotenv.2015.11.166 eng eng info:eu-repo/semantics/altIdentifier/pmid/26674690 info:eu-repo/semantics/altIdentifier/wos/WOS:000369491500066 volume:544 firstpage:606 lastpage:616 numberofpages:11 journal:SCIENCE OF THE TOTAL ENVIRONMENT http://hdl.handle.net/10278/3680486 doi:10.1016/j.scitotenv.2015.11.166 info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-84949844474 www.elsevier.com/locate/scitotenv info:eu-repo/semantics/openAccess Aerosol Antarctica Biomass burning Levoglucosan Phenolic compound Environmental Chemistry Pollution Waste Management and Disposal Environmental Engineering Settore CHIM/01 - Chimica Analitica info:eu-repo/semantics/article 2016 ftuniveneziairis https://doi.org/10.1016/j.scitotenv.2015.11.166 2024-03-21T18:13:58Z Due to its isolated location, Antarctica is a natural laboratory for studying atmospheric aerosols and pollution in remote areas. Here, we determined levoglucosan and phenolic compounds (PCs) at diverse Antarctic sites: on the plateau, a coastal station and during an oceanographic cruise. Levoglucosan and PCs reached the Antarctic plateau where they were observed in accumulation mode aerosols (with median levoglucosan concentrations of 6.4pgm-3 and 4.1pgm-3, and median PC concentrations of 15.0pgm-3 and 7.3pgm-3). Aged aerosols arrived at the coastal site through katabatic circulation with the majority of the levoglucosan mass distributed on larger particulates (24.8pgm-3), while PCs were present in fine particles (34.0pgm-3). The low levoglucosan/PC ratios in Antarctic aerosols suggest that biomass burning aerosols only had regional, rather than local, sources. General acid/aldehyde ratios were lower at the coastal site than on the plateau. Levoglucosan and PCs determined during the oceanographic cruise were 37.6pgm-3 and 58.5pgm-3 respectively. Unlike levoglucosan, which can only be produced by biomass burning, PCs have both biomass burning and other sources. Our comparisons of these two types of compounds across a range of Antarctic marine, coastal, and plateau sites demonstrate that local marine sources dominate Antarctic PC concentrations. Article in Journal/Newspaper Antarc* Antarctic Antarctica Università Ca’ Foscari Venezia: ARCA (Archivio Istituzionale della Ricerca) Antarctic The Antarctic Science of The Total Environment 544 606 616 |
institution |
Open Polar |
collection |
Università Ca’ Foscari Venezia: ARCA (Archivio Istituzionale della Ricerca) |
op_collection_id |
ftuniveneziairis |
language |
English |
topic |
Aerosol Antarctica Biomass burning Levoglucosan Phenolic compound Environmental Chemistry Pollution Waste Management and Disposal Environmental Engineering Settore CHIM/01 - Chimica Analitica |
spellingShingle |
Aerosol Antarctica Biomass burning Levoglucosan Phenolic compound Environmental Chemistry Pollution Waste Management and Disposal Environmental Engineering Settore CHIM/01 - Chimica Analitica ZANGRANDO, Roberta BARBARO, ELENA VECCHIATO, MARCO KEHRWALD, NATALIE MARIE BARBANTE, Carlo GAMBARO, Andrea Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols |
topic_facet |
Aerosol Antarctica Biomass burning Levoglucosan Phenolic compound Environmental Chemistry Pollution Waste Management and Disposal Environmental Engineering Settore CHIM/01 - Chimica Analitica |
description |
Due to its isolated location, Antarctica is a natural laboratory for studying atmospheric aerosols and pollution in remote areas. Here, we determined levoglucosan and phenolic compounds (PCs) at diverse Antarctic sites: on the plateau, a coastal station and during an oceanographic cruise. Levoglucosan and PCs reached the Antarctic plateau where they were observed in accumulation mode aerosols (with median levoglucosan concentrations of 6.4pgm-3 and 4.1pgm-3, and median PC concentrations of 15.0pgm-3 and 7.3pgm-3). Aged aerosols arrived at the coastal site through katabatic circulation with the majority of the levoglucosan mass distributed on larger particulates (24.8pgm-3), while PCs were present in fine particles (34.0pgm-3). The low levoglucosan/PC ratios in Antarctic aerosols suggest that biomass burning aerosols only had regional, rather than local, sources. General acid/aldehyde ratios were lower at the coastal site than on the plateau. Levoglucosan and PCs determined during the oceanographic cruise were 37.6pgm-3 and 58.5pgm-3 respectively. Unlike levoglucosan, which can only be produced by biomass burning, PCs have both biomass burning and other sources. Our comparisons of these two types of compounds across a range of Antarctic marine, coastal, and plateau sites demonstrate that local marine sources dominate Antarctic PC concentrations. |
author2 |
Zangrando, Roberta Barbaro, Elena Vecchiato, Marco Kehrwald, NATALIE MARIE Barbante, Carlo Gambaro, Andrea |
format |
Article in Journal/Newspaper |
author |
ZANGRANDO, Roberta BARBARO, ELENA VECCHIATO, MARCO KEHRWALD, NATALIE MARIE BARBANTE, Carlo GAMBARO, Andrea |
author_facet |
ZANGRANDO, Roberta BARBARO, ELENA VECCHIATO, MARCO KEHRWALD, NATALIE MARIE BARBANTE, Carlo GAMBARO, Andrea |
author_sort |
ZANGRANDO, Roberta |
title |
Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols |
title_short |
Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols |
title_full |
Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols |
title_fullStr |
Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols |
title_full_unstemmed |
Levoglucosan and phenols in Antarctic marine, coastal and plateau aerosols |
title_sort |
levoglucosan and phenols in antarctic marine, coastal and plateau aerosols |
publishDate |
2016 |
url |
http://hdl.handle.net/10278/3680486 https://doi.org/10.1016/j.scitotenv.2015.11.166 |
geographic |
Antarctic The Antarctic |
geographic_facet |
Antarctic The Antarctic |
genre |
Antarc* Antarctic Antarctica |
genre_facet |
Antarc* Antarctic Antarctica |
op_relation |
info:eu-repo/semantics/altIdentifier/pmid/26674690 info:eu-repo/semantics/altIdentifier/wos/WOS:000369491500066 volume:544 firstpage:606 lastpage:616 numberofpages:11 journal:SCIENCE OF THE TOTAL ENVIRONMENT http://hdl.handle.net/10278/3680486 doi:10.1016/j.scitotenv.2015.11.166 info:eu-repo/semantics/altIdentifier/scopus/2-s2.0-84949844474 www.elsevier.com/locate/scitotenv |
op_rights |
info:eu-repo/semantics/openAccess |
op_doi |
https://doi.org/10.1016/j.scitotenv.2015.11.166 |
container_title |
Science of The Total Environment |
container_volume |
544 |
container_start_page |
606 |
op_container_end_page |
616 |
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1796300400988520448 |