The Longyearbyen CO2 Lab: Fluid communication in reservoir and caprock

• Published in: International Journal of Greenhouse Gas Control
• Main Authors: Huq, Farhana, Smalley, P. Craig, Mørkved, Pål Tore, Johansen, Ingar, Yarushina, Viktoriya, Johansen, Harald
• Format: Article in Journal/Newspaper
• Language: English
• Published: Elsevier 2017
• Subjects: CO2 storage; Sr isotope; C isotope; Site characterization; Fluid flow; Large-scale CCS; Caprock; Longyearbyen; Norway; Svalbard; permafrost; Spitsbergen
• Online Access: https://hdl.handle.net/1956/17671; https://doi.org/10.1016/j.ijggc.2017.05.005

The Longyearbyen CO2 Lab of Svalbard, Norway was established to estimate the potential for geological carbon sequestration at Spitsbergen. Several monitoring wells were drilled in and around the planned CO2 injection site. These revealed a Triassic to Cretaceous stratigraphy consisting of (from top to bottom) a zone of permafrost, the aquifer, the caprock shale, and the upper, middle and lower reservoir. This paper uses two tools to investigate fluid communication within and between these entities: 87Sr/86Sr of formation waters extracted from cores using the residual salt analysis (RSA) method, and the δ13C of gases, principally methane and CO2, degassed from core samples. The Sr RSA data reveal that the upper reservoir rocks have very constant formation water 87Sr/86Sr (0.7130) in wells several kilometres apart, suggesting good lateral communication on a geological timescale. However, there is a distinct barrier to vertical communication within the middle reservoir, indicated by a step change in 87Sr/86Sr (0.7130–0.7112), corresponding to thin but presumably laterally extensive (>1.5 km) lagoonal mudrocks. The aquifer, which shows a gradient in 87Sr/86Sr, is also interpreted to have some degree of vertical internal communication on a geological time scale. The caprock shale shows large-scale (over 350 m) smooth vertical gradient in 87Sr/86Sr (0.7200-0.7130). This is indicative of an ongoing mixing process between high- 87Sr/86Sr waters within the caprock and lower- 87Sr/86Sr waters in the underlying reservoir. Diffusion and flow modelling of the Sr data suggest that at some time in the past, shale fluid transport properties were enhanced by the formation of temporary pressure escape features (fractures or chimneys) during deep burial and uplift, or cycles of glaciation. Nevertheless, the smooth compositional gradient in the caprock indicates that fluid mixing has subsequently taken place slowly, dominated by diffusion. This interpretation is supported by the gas isotope data, where systematic variations in ...