Simultaneous measurements of aerosol size distributions at three sites in the European high Arctic

• Published in: Atmospheric Chemistry and Physics
• Main Authors: Dall'Osto, Manuel, Beddows, David C. S., Tunved, Peter, Harrison, Roy M., Lupi, Angelo, Vitale, Vito, Becagli, Silvia, Traversi, Rita, Park, Ki-Tae, Yoon, Young Jun, Massling, Andreas, Skov, Henrik, Lange, Robert, Ström, Johan, Krejci, Radovan
• Format: Article in Journal/Newspaper
• Language: English
• Published: 2019
• Subjects: AMMONIA; DICARBOXYLIC-ACIDS; NY-ALESUND; PARTICLE FORMATION; PHYTOPLANKTON BLOOMS; SEA-ICE; SOURCE APPORTIONMENT; STATISTICAL-ANALYSIS; SUBMICRON AEROSOL; SUMMER BOUNDARY-LAYER; Aitken; Arctic; Greenland; Station Nord; Svalbard; Svalbard Archipelago; Phytoplankton; Sea ice
• Online Access: https://pure.au.dk/portal/da/publications/simultaneous-measurements-of-aerosol-size-distributions-at-three-sites-in-the-european-high-arctic(bade8477-ff5c-49f3-bcb0-74335e58cafd).html; https://doi.org/10.5194/acp-19-7377-2019; http://www.scopus.com/inward/record.url?scp=85066856641&partnerID=8YFLogxK

Aerosols are an integral part of the Arctic climate system due to their direct interaction with radiation and indirect interaction through cloud formation. Understanding aerosol size distributions and their dynamics is crucial for the ability to predict these climate relevant effects. When of favourable size and composition, both long-rangetransported-and locally formed particles-may serve as cloud condensation nuclei (CCN). Small changes of composition or size may have a large impact on the low CCN concentrations currently characteristic of the Arctic environment. We present a cluster analysis of particle size distributions (PSDs; size range 8-500 nm) simultaneously collected from three high Arctic sites during a 3-year period (2013-2015). Two sites are located in the Svalbard archipelago: Zeppelin research station (ZEP; 474 m above ground) and the nearby Gruvebadet Observatory (GRU; about 2 km distance from Zeppelin, 67 m above ground). The third site (Villum Research Station at Station Nord, VRS; 30 m above ground) is 600 km west-northwest of Zeppelin, at the tip of northeastern Greenland. The GRU site is included in an inter-site comparison for the first time. K-means cluster analysis provided eight specific aerosol categories, further combined into broad PSD classes with similar characteristics, namely pristine low concentrations (12 %-14 % occurrence), new particle formation (16 %-32 %), Aitken (21 %-35 %) and accumulation (20 %-50 %). Confined for longer time periods by consolidated pack sea ice regions, the Greenland site GRU shows PSDs with lower ultrafine-mode aerosol concentrations during summer but higher accumulation-mode aerosol concentrations during winter, relative to the Svalbard sites. By association with chemical composition and cloud condensation nuclei properties, further conclusions can be derived. Three distinct types of accumulation-mode aerosol are observed during winter months. These are associated with sea spray (largest detectable sizes, > 400 nm), Arctic haze (main mode at 150 nm) ...