Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study
Depending on the magnitude of their eruptions, volcanoes impact the atmosphere at various temporal and spatial scales. The volcanic source remains a major unknown to rigorously assess these impacts. At the scale of an eruption, the limited knowledge of source parameters, including time-variations of...
Published in: | Atmospheric Chemistry and Physics |
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Format: | Article in Journal/Newspaper |
Language: | English |
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2013
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Online Access: | https://doi.org/10.5194/acp-13-8569-2013 https://hal.archives-ouvertes.fr/hal-00799237/file/acp-13-8569-2013.pdf https://hal.archives-ouvertes.fr/hal-00799237 |
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geo info Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
topic_facet |
geo info |
description |
Depending on the magnitude of their eruptions, volcanoes impact the atmosphere at various temporal and spatial scales. The volcanic source remains a major unknown to rigorously assess these impacts. At the scale of an eruption, the limited knowledge of source parameters, including time-variations of erupted mass flux and emission profile, currently represents the greatest issue that limits the reliability of volcanic cloud forecasts. Today, a growing number of satellite and remote sensing observations of distant plumes are becoming available, bringing indirect information on these source terms. Here, we develop an inverse modeling approach combining satellite observations of the volcanic plume with an Eulerian regional chemistry-transport model (CHIMERE) to better characterise the volcanic SO2 emissions during an eruptive crisis. The May 2010 eruption of Eyjafjallajökull is a perfect case-study to apply this method as the volcano emitted substantial amounts of SO2 during more than a month. We take advantage of the SO2 column amounts provided by a vast set of IASI (Infrared Atmospheric Sounding Interferometer) satellite images to reconstruct retrospectively the time-series of the mid-tropospheric SO2 flux emitted by the volcano with a temporal resolution of ~2 h, spanning the period from 1 to 12 May 2010. The initialisation of chemistry-transport modelling with this reconstructed source allows for a reliable simulation of the evolution of the long-lived tropospheric SO2 cloud over thousands of kilometres. Heterogeneities within the plume, which mainly result from the temporal variability of the emissions, are correctly tracked over a time scale of a week. The robustness of our approach is also demonstrated by the broad similarities between the SO2 flux history determined by this study and the ash discharge behaviour estimated by other means during the phases of high explosive activity at Eyjafjallajökull in May 2010. Finally, we show how a sequential IASI data assimilation allows for a substantial improvement in ... |
author2 |
Laboratoire de Météorologie Dynamique (UMR 8539) (LMD) Département des Géosciences - ENS Paris École normale supérieure - Paris (ENS Paris) Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris) Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-École des Ponts ParisTech (ENPC)-École polytechnique (X)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Pierre et Marie Curie - Paris 6 (UPMC) Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique Université libre de Bruxelles (ULB) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) |
format |
Article in Journal/Newspaper |
author |
Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François |
author_facet |
Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François |
author_sort |
Boichu, Marie |
title |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_short |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_full |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_fullStr |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_full_unstemmed |
Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study |
title_sort |
inverting for volcanic so2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 eyjafjallajökull eruption case-study |
publisher |
HAL CCSD |
publishDate |
2013 |
url |
https://doi.org/10.5194/acp-13-8569-2013 https://hal.archives-ouvertes.fr/hal-00799237/file/acp-13-8569-2013.pdf https://hal.archives-ouvertes.fr/hal-00799237 |
genre |
Eyjafjallajökull |
genre_facet |
Eyjafjallajökull |
op_source |
Hyper Article en Ligne - Sciences de l'Homme et de la Société ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics Atmospheric Chemistry and Physics, European Geosciences Union, 2013, 13 (17), pp.8569-8584. ⟨10.5194/acp-13-8569-2013⟩ |
op_relation |
hal-00799237 doi:10.5194/acp-13-8569-2013 10670/1.y0q3nc https://hal.archives-ouvertes.fr/hal-00799237/file/acp-13-8569-2013.pdf https://hal.archives-ouvertes.fr/hal-00799237 |
op_doi |
https://doi.org/10.5194/acp-13-8569-2013 |
container_title |
Atmospheric Chemistry and Physics |
container_volume |
13 |
container_issue |
17 |
container_start_page |
8569 |
op_container_end_page |
8584 |
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1766405350593921024 |
spelling |
fttriple:oai:gotriple.eu:10670/1.y0q3nc 2023-05-15T16:09:28+02:00 Inverting for volcanic SO2 flux at high temporal resolution using spaceborne plume imagery and chemistry-transport modelling: the 2010 Eyjafjallajökull eruption case-study Boichu, Marie Menut, Laurent Khvorostyanov, Dmitry Clarisse, L. Clerbaux, Cathy Turquety, Solène Coheur, Pierre-François Laboratoire de Météorologie Dynamique (UMR 8539) (LMD) Département des Géosciences - ENS Paris École normale supérieure - Paris (ENS Paris) Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris) Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-École des Ponts ParisTech (ENPC)-École polytechnique (X)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Pierre et Marie Curie - Paris 6 (UPMC) Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique Université libre de Bruxelles (ULB) TROPO - LATMOS Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS) Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS) 2013-01-01 https://doi.org/10.5194/acp-13-8569-2013 https://hal.archives-ouvertes.fr/hal-00799237/file/acp-13-8569-2013.pdf https://hal.archives-ouvertes.fr/hal-00799237 en eng HAL CCSD European Geosciences Union hal-00799237 doi:10.5194/acp-13-8569-2013 10670/1.y0q3nc https://hal.archives-ouvertes.fr/hal-00799237/file/acp-13-8569-2013.pdf https://hal.archives-ouvertes.fr/hal-00799237 Hyper Article en Ligne - Sciences de l'Homme et de la Société ISSN: 1680-7316 EISSN: 1680-7324 Atmospheric Chemistry and Physics Atmospheric Chemistry and Physics, European Geosciences Union, 2013, 13 (17), pp.8569-8584. ⟨10.5194/acp-13-8569-2013⟩ geo info Journal Article https://vocabularies.coar-repositories.org/resource_types/c_6501/ 2013 fttriple https://doi.org/10.5194/acp-13-8569-2013 2023-01-22T18:33:11Z Depending on the magnitude of their eruptions, volcanoes impact the atmosphere at various temporal and spatial scales. The volcanic source remains a major unknown to rigorously assess these impacts. At the scale of an eruption, the limited knowledge of source parameters, including time-variations of erupted mass flux and emission profile, currently represents the greatest issue that limits the reliability of volcanic cloud forecasts. Today, a growing number of satellite and remote sensing observations of distant plumes are becoming available, bringing indirect information on these source terms. Here, we develop an inverse modeling approach combining satellite observations of the volcanic plume with an Eulerian regional chemistry-transport model (CHIMERE) to better characterise the volcanic SO2 emissions during an eruptive crisis. The May 2010 eruption of Eyjafjallajökull is a perfect case-study to apply this method as the volcano emitted substantial amounts of SO2 during more than a month. We take advantage of the SO2 column amounts provided by a vast set of IASI (Infrared Atmospheric Sounding Interferometer) satellite images to reconstruct retrospectively the time-series of the mid-tropospheric SO2 flux emitted by the volcano with a temporal resolution of ~2 h, spanning the period from 1 to 12 May 2010. The initialisation of chemistry-transport modelling with this reconstructed source allows for a reliable simulation of the evolution of the long-lived tropospheric SO2 cloud over thousands of kilometres. Heterogeneities within the plume, which mainly result from the temporal variability of the emissions, are correctly tracked over a time scale of a week. The robustness of our approach is also demonstrated by the broad similarities between the SO2 flux history determined by this study and the ash discharge behaviour estimated by other means during the phases of high explosive activity at Eyjafjallajökull in May 2010. Finally, we show how a sequential IASI data assimilation allows for a substantial improvement in ... Article in Journal/Newspaper Eyjafjallajökull Unknown Atmospheric Chemistry and Physics 13 17 8569 8584 |