Air pollution impacts due to petroleum extraction in the Norwegian Sea during the ACCESS aircraft campaign

• Published in: Elementa: Science of the Anthropocene
• Main Authors: Tuccella, Paolo, Thomas, Jennie L., Law, Kathy S., Raut, Jean-Christophe, Marelle, Louis, Roiger, Anke, Weinzierl, B., Denier Van Der Gon, H., Schlager, H., Onishi, Tatsuo
• Other Authors: NUMTECH, Laboratoire de Météorologie Dynamique (UMR 8539) (LMD), Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-École des Ponts ParisTech (ENPC)-École polytechnique (X)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Pierre et Marie Curie - Paris 6 (UPMC), TROPO - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Center for International Climate and Environmental Research Oslo (CICERO), University of Oslo (UiO), DLR Institut für Physik der Atmosphäre (IPA), Deutsches Zentrum für Luft- und Raumfahrt Oberpfaffenhofen-Wessling (DLR), Aerosol Physics and Environmental Physics Vienna, University of Vienna Vienna, TNO Climate, Air and Sustainability Utrecht, The Netherlands Organisation for Applied Scientific Research (TNO), European Union, CNRS (Chantier Arctique PARCS), European Project: 265863,EC:FP7:TPT,FP7-OCEAN-2010,ACCESS(2011)
• Format: Article in Journal/Newspaper
• Language: English
• Published: HAL CCSD 2017
• Subjects: Arctic pollution; air quality modeling; Norwegian Sea oil/gas extraction; oil/gas pollution; oil/gas emissions; envir; geo; Arctic; Norwegian Sea; black carbon; Global warming
• Online Access: https://doi.org/10.1525/elementa.124; https://hal-insu.archives-ouvertes.fr/insu-01538609/file/tuccella.pdf; https://hal-insu.archives-ouvertes.fr/insu-01538609

International audience Emissions from oil/gas extraction activities in the Arctic are already important in certain regions and may increase as global warming opens up new opportunities for industrial development. Emissions from oil/gas extraction are sources of air pollutants, but large uncertainties exist with regard to their amounts and composition. In this study, we focus on detailed investigation of emissions from oil/gas extraction in the Norwegian Sea combining measurements from the EU ACCESS aircraft campaign in July 2012 and regional chemical transport modeling. The goal is to (1) evaluate emissions from petroleum extraction activities and (2) investigate their impact on atmospheric composition over the Norwegian Sea. Numerical simulations include emissions for permanently operating offshore facilities from two datasets: the TNO-MACC inventory and emissions reported by Norwegian Environment Agency (NEA). It was necessary to additionally estimate primary aerosol emissions using reported emission factors since these emissions are not included in the inventories for our sites. Model runs with the TNO-MACC emissions are unable to reproduce observations close to the facilities. Runs using the NEA emissions more closely reproduce the observations although emissions from mobile facilities are missing from this inventory. Measured plumes suggest they are a significant source of pollutants, in particular NOx and aerosols. Sensitivities to NOx and NMVOC emissions show that, close to the platforms, O3 is sensitive to NOx emissions and is much less sensitive to NMVOC emissions. O3 destruction, via reaction with NO, dominates very close to the platforms. Far from the platforms, oil/gas facility emissions result in an average daytime O3 enhancement of +2% at the surface. Larger enhancements are predicted at noon ranging from +7% at the surface to +15% at 600 m. Black carbon is the aerosol species most strongly influenced by petroleum extraction emissions. The results highlight significant uncertainties in emissions ...