Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling

Destabilization of intrapermafrost gas hydrate is one possible reason for methane emission on the Arctic shelf. The formation of these intrapermafrost gas hydrates could occur almost simultaneously with the permafrost sediments due to the occurrence of a hydrate stability zone after sea regression a...

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Published in:Geosciences
Main Authors: Chuvilin, Evgeny Mikhaylovich, Ekimova, Valentina, Bukhanov, Boris Aleksandrovich, Grebenkin, Sergey Igorevich, Shakhova, Nataljya Evgenjevna, Semiletov, Igor Petrovich
Format: Article in Journal/Newspaper
Language:English
Published: MDPI AG 2019
Subjects:
Online Access:http://earchive.tpu.ru/handle/11683/64910
https://doi.org/10.3390/geosciences9040188
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spelling fttomskpuniv:oai:earchive.tpu.ru:11683/64910 2023-05-15T14:25:49+02:00 Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling Chuvilin, Evgeny Mikhaylovich Ekimova, Valentina Bukhanov, Boris Aleksandrovich Grebenkin, Sergey Igorevich Shakhova, Nataljya Evgenjevna Semiletov, Igor Petrovich 2019 application/pdf http://earchive.tpu.ru/handle/11683/64910 https://doi.org/10.3390/geosciences9040188 en eng MDPI AG Geosciences. 2019. Vol. 9, iss. 4 Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling / E. M. Chuvilin, V. V. Ekimova, B. A. Bukhanov [et al.] // Geosciences. — 2019. — Vol. 9, iss. 4. — [188, 18 p.]. http://earchive.tpu.ru/handle/11683/64910 doi:10.3390/geosciences9040188 info:eu-repo/semantics/openAccess Attribution-NonCommercial 4.0 International https://creativecommons.org/licenses/by-nc/4.0/ CC-BY-NC Geosciences арктический шельф вечная мерзлота газовые гидраты arctic shelf permafrost gas hydrate temperature increase hydrate dissociation methane emission environmental impact geohazard Article info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion 2019 fttomskpuniv https://doi.org/10.3390/geosciences9040188 2021-03-30T16:27:56Z Destabilization of intrapermafrost gas hydrate is one possible reason for methane emission on the Arctic shelf. The formation of these intrapermafrost gas hydrates could occur almost simultaneously with the permafrost sediments due to the occurrence of a hydrate stability zone after sea regression and the subsequent deep cooling and freezing of sediments. The top of the gas hydrate stability zone could exist not only at depths of 200–250 m, but also higher due to local pressure increase in gas-saturated horizons during freezing. Formed at a shallow depth, intrapermafrost gas hydrates could later be preserved and transform into a metastable (relict) state. Under the conditions of submarine permafrost degradation, exactly relict hydrates located above the modern gas hydrate stability zone will, first of all, be involved in the decomposition process caused by negative temperature rising, permafrost thawing, and sediment salinity increasing. That’s why special experiments were conducted on the interaction of frozen sandy sediments containing relict methane hydrates with salt solutions of different concentrations at negative temperatures to assess the conditions of intrapermafrost gas hydrates dissociation. Experiments showed that the migration of salts into frozen hydrate-containing sediments activates the decomposition of pore gas hydrates and increase the methane emission. These results allowed for an understanding of the mechanism of massive methane release from bottom sediments of the East Siberian Arctic shelf. Article in Journal/Newspaper Arctic Arctic permafrost вечная мерзлота Tomsk Polytechnic University (TPU): Electronic Archive Arctic Geosciences 9 4 188
institution Open Polar
collection Tomsk Polytechnic University (TPU): Electronic Archive
op_collection_id fttomskpuniv
language English
topic арктический шельф
вечная мерзлота
газовые гидраты
arctic shelf
permafrost
gas hydrate
temperature increase
hydrate dissociation
methane emission
environmental impact
geohazard
spellingShingle арктический шельф
вечная мерзлота
газовые гидраты
arctic shelf
permafrost
gas hydrate
temperature increase
hydrate dissociation
methane emission
environmental impact
geohazard
Chuvilin, Evgeny Mikhaylovich
Ekimova, Valentina
Bukhanov, Boris Aleksandrovich
Grebenkin, Sergey Igorevich
Shakhova, Nataljya Evgenjevna
Semiletov, Igor Petrovich
Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling
topic_facet арктический шельф
вечная мерзлота
газовые гидраты
arctic shelf
permafrost
gas hydrate
temperature increase
hydrate dissociation
methane emission
environmental impact
geohazard
description Destabilization of intrapermafrost gas hydrate is one possible reason for methane emission on the Arctic shelf. The formation of these intrapermafrost gas hydrates could occur almost simultaneously with the permafrost sediments due to the occurrence of a hydrate stability zone after sea regression and the subsequent deep cooling and freezing of sediments. The top of the gas hydrate stability zone could exist not only at depths of 200–250 m, but also higher due to local pressure increase in gas-saturated horizons during freezing. Formed at a shallow depth, intrapermafrost gas hydrates could later be preserved and transform into a metastable (relict) state. Under the conditions of submarine permafrost degradation, exactly relict hydrates located above the modern gas hydrate stability zone will, first of all, be involved in the decomposition process caused by negative temperature rising, permafrost thawing, and sediment salinity increasing. That’s why special experiments were conducted on the interaction of frozen sandy sediments containing relict methane hydrates with salt solutions of different concentrations at negative temperatures to assess the conditions of intrapermafrost gas hydrates dissociation. Experiments showed that the migration of salts into frozen hydrate-containing sediments activates the decomposition of pore gas hydrates and increase the methane emission. These results allowed for an understanding of the mechanism of massive methane release from bottom sediments of the East Siberian Arctic shelf.
format Article in Journal/Newspaper
author Chuvilin, Evgeny Mikhaylovich
Ekimova, Valentina
Bukhanov, Boris Aleksandrovich
Grebenkin, Sergey Igorevich
Shakhova, Nataljya Evgenjevna
Semiletov, Igor Petrovich
author_facet Chuvilin, Evgeny Mikhaylovich
Ekimova, Valentina
Bukhanov, Boris Aleksandrovich
Grebenkin, Sergey Igorevich
Shakhova, Nataljya Evgenjevna
Semiletov, Igor Petrovich
author_sort Chuvilin, Evgeny Mikhaylovich
title Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling
title_short Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling
title_full Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling
title_fullStr Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling
title_full_unstemmed Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling
title_sort role of salt migration in destabilization of intra permafrost hydrates in the arctic shelf: experimental modeling
publisher MDPI AG
publishDate 2019
url http://earchive.tpu.ru/handle/11683/64910
https://doi.org/10.3390/geosciences9040188
geographic Arctic
geographic_facet Arctic
genre Arctic
Arctic
permafrost
вечная мерзлота
genre_facet Arctic
Arctic
permafrost
вечная мерзлота
op_source Geosciences
op_relation Geosciences. 2019. Vol. 9, iss. 4
Role of Salt Migration in Destabilization of Intra Permafrost Hydrates in the Arctic Shelf: Experimental Modeling / E. M. Chuvilin, V. V. Ekimova, B. A. Bukhanov [et al.] // Geosciences. — 2019. — Vol. 9, iss. 4. — [188, 18 p.].
http://earchive.tpu.ru/handle/11683/64910
doi:10.3390/geosciences9040188
op_rights info:eu-repo/semantics/openAccess
Attribution-NonCommercial 4.0 International
https://creativecommons.org/licenses/by-nc/4.0/
op_rightsnorm CC-BY-NC
op_doi https://doi.org/10.3390/geosciences9040188
container_title Geosciences
container_volume 9
container_issue 4
container_start_page 188
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