Reconstruction of flux and altitude of volcanic SO2 emissions from IASIsatellite observations: implications for volcanological and atmosphericalstudies.

• Main Authors: Boichu, Marie, Clarisse, Lieven, Péré, Jean-Christophe, Herbin, Hervé, Goloub, Philippe, Thieuleux, François, Khvorostyanov, Dmitry, Ducos, Fabrice, Winiarek, Victor, Clerbaux, Cathy, Tanré, Didier
• Other Authors: Laboratoire d’Optique Atmosphérique - UMR 8518 (LOA), Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique, Université libre de Bruxelles (ULB), Interactions Aérosols Rayonnement (IAR), Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Météorologie Dynamique (UMR 8539) (LMD), Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X), Institut Polytechnique de Paris (IP Paris)-Institut Polytechnique de Paris (IP Paris)-École des Ponts ParisTech (ENPC)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL), TROPO - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)
• Format: Conference Object
• Language: English
• Published: HAL CCSD 2016
• Subjects: [PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph]; Eyjafjallajökull; Iceland
• Online Access: https://insu.hal.science/insu-01306362

International audience Volcanic SO2 degassing is a crucial indicator of the sub-surface volcanic activity, which is widelyused today for volcano monitoring and hazard assessment purposes. Volcanic SO2 is also importantregarding atmospherical studies. More easily detectable from space, SO2 can be used as a proxy ofthe presence of ash to anticipate air traffic issues caused by explosive eruptions. Moreover, volcanicSO2 strongly impacts air quality but also climate following its conversion to radiatively-activesulphate aerosols. However, the accurate assessment of these various impacts is currently hamperedby the poor knowledge of volcanic SO2 emissions, which can substantially vary with time, in termsof flux and altitude.To fulfil this need, we propose a strategy relying on satellite observations, which consequently allowsfor monitoring the eruptive activity of any remote volcano. The method consists in assimilatingsnapshots of the SO2 load, provided every ~12 hours by IASI, in an inversion scheme that involvesthe use of a chemistry-transport model to describe the dispersion of SO2 released in the atmosphere.Applied on Eyjafjallajökull (Iceland) and Etna (Italy) eruption case-studies, this procedure allows forretrospectively reconstructing both the flux and altitude of the SO2 emissions with an hourlyresolution. We show the improvement gained in the simulations and forecasts of the location andmass load of volcanic SO2 clouds using such a detailed reconstruction of emissions.For calibration-validation purpose, we compared our satellite-derived time-series of the SO2 fluxwith ground-based observations available on Etna. This comparison indicates a good agreementduring ash-poor phases of the eruption. However, large discrepancies are observed during the ashrichparoxysmal phase as a result of enhanced plume opacity affecting ground-based ultravioletspectroscopic retrievals. Therefore, the SO2 emission rate derived from the ground is underestimatedby almost one order of magnitude. This result calls for the necessity ...