An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result
The amount of carbon dioxide (CO 2 ) in the atmosphere has increased in the past 60 years and the technology of carbon capture and storage (CCS) has recently been extensively studied. One of the strategies of CCS is to directly inject a high dissolved inorganic carbon (DIC) concentration (or high pa...
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ftrepec:oai:RePEc:gam:jsusta:v:10:y:2018:i:4:p:1174-:d:141001 2024-04-14T08:17:42+00:00 An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result Wei-Jen Huang Kai-Jung Kao Li-Lian Liu Chi-Wen Liao Yin-Lung Han https://www.mdpi.com/2071-1050/10/4/1174/pdf https://www.mdpi.com/2071-1050/10/4/1174/ unknown https://www.mdpi.com/2071-1050/10/4/1174/pdf https://www.mdpi.com/2071-1050/10/4/1174/ article ftrepec 2024-03-19T10:30:12Z The amount of carbon dioxide (CO 2 ) in the atmosphere has increased in the past 60 years and the technology of carbon capture and storage (CCS) has recently been extensively studied. One of the strategies of CCS is to directly inject a high dissolved inorganic carbon (DIC) concentration (or high partial pressure of carbon dioxide, p CO 2 ) solution into the ocean. However, the carbonate dynamics and air-sea gas exchange are usually neglected in a CCS strategy. This study assesses the effect of a DIC-solution injection by using a simple two end-member model to simulate the variation of pH, DIC, total alkalinity (TA) and p CO 2 between the river and sea mixing process for the Danshuei River estuary and Hoping River in Taiwan. We observed that the DIC-solution injection can contribute to ocean acidification and can also lead the p CO 2 value to change from being undersaturated to oversaturated (with respect to the atmospheric CO 2 level). Our model result also showed that the maximum Revelle factors (Δ[CO 2 ]/[CO 2 ])/(Δ[DIC]/[DIC]) among varied pH values (6–9) and DIC concentrations (0.5–3.5 mmol kg −1 ) were between pH 8.3 and 8.5 in fresh water and were between 7.3 and 7.5 in waters with a salinity of 35, reflecting the changing efficiency of dissolving CO 2 gas into the DIC solution and the varying stability of this desired DIC solution. Finally, we suggest this uncoupled Revelle factor between fresh and salty water should be considered in the (anthropogenic) carbonate chemical weathering on a decade to century scale. carbon cycle; ocean acidification; air-sea gas exchange; CO 2 CCS Article in Journal/Newspaper Ocean acidification RePEc (Research Papers in Economics) |
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RePEc (Research Papers in Economics) |
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The amount of carbon dioxide (CO 2 ) in the atmosphere has increased in the past 60 years and the technology of carbon capture and storage (CCS) has recently been extensively studied. One of the strategies of CCS is to directly inject a high dissolved inorganic carbon (DIC) concentration (or high partial pressure of carbon dioxide, p CO 2 ) solution into the ocean. However, the carbonate dynamics and air-sea gas exchange are usually neglected in a CCS strategy. This study assesses the effect of a DIC-solution injection by using a simple two end-member model to simulate the variation of pH, DIC, total alkalinity (TA) and p CO 2 between the river and sea mixing process for the Danshuei River estuary and Hoping River in Taiwan. We observed that the DIC-solution injection can contribute to ocean acidification and can also lead the p CO 2 value to change from being undersaturated to oversaturated (with respect to the atmospheric CO 2 level). Our model result also showed that the maximum Revelle factors (Δ[CO 2 ]/[CO 2 ])/(Δ[DIC]/[DIC]) among varied pH values (6–9) and DIC concentrations (0.5–3.5 mmol kg −1 ) were between pH 8.3 and 8.5 in fresh water and were between 7.3 and 7.5 in waters with a salinity of 35, reflecting the changing efficiency of dissolving CO 2 gas into the DIC solution and the varying stability of this desired DIC solution. Finally, we suggest this uncoupled Revelle factor between fresh and salty water should be considered in the (anthropogenic) carbonate chemical weathering on a decade to century scale. carbon cycle; ocean acidification; air-sea gas exchange; CO 2 CCS |
format |
Article in Journal/Newspaper |
author |
Wei-Jen Huang Kai-Jung Kao Li-Lian Liu Chi-Wen Liao Yin-Lung Han |
spellingShingle |
Wei-Jen Huang Kai-Jung Kao Li-Lian Liu Chi-Wen Liao Yin-Lung Han An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result |
author_facet |
Wei-Jen Huang Kai-Jung Kao Li-Lian Liu Chi-Wen Liao Yin-Lung Han |
author_sort |
Wei-Jen Huang |
title |
An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result |
title_short |
An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result |
title_full |
An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result |
title_fullStr |
An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result |
title_full_unstemmed |
An Assessment of Direct Dissolved Inorganic Carbon Injection to the Coastal Region: A Model Result |
title_sort |
assessment of direct dissolved inorganic carbon injection to the coastal region: a model result |
url |
https://www.mdpi.com/2071-1050/10/4/1174/pdf https://www.mdpi.com/2071-1050/10/4/1174/ |
genre |
Ocean acidification |
genre_facet |
Ocean acidification |
op_relation |
https://www.mdpi.com/2071-1050/10/4/1174/pdf https://www.mdpi.com/2071-1050/10/4/1174/ |
_version_ |
1796316946351783936 |